Mechanism of phthalic anhydride formation in the oxidation of n-pentane on a vanadium-phosphorus oxide catalystKinetics and Catalysis - - 2006
V. A. Zazhigalov, E. V. Cheburakova, M. Gansior, J. Stoch
The reaction paths of product formation in the partial oxidation of n-pentane on
vanadium-phosphorus oxide (VPO) and VPO-Bi catalysts are considered. The
condensed products of n-pentane oxidation were analyzed by chromatography-mass
spectrometry, and the presence of C4 rather than C5 unsaturated hydrocarbons was
detected. It was found that the concentration of phthalic anhydride in the
products in... hiện toàn bộ
Kinetic parameters of the cyclization and decyclization reactions of nitrogen- and oxygen-containing radicalsKinetics and Catalysis - Tập 46 - Trang 1-9 - 2005
T. G. Denisova, E. T. Denisov
The intersecting parabolas model is used to analyze experimental data for the
following radical cyclization and decyclization reactions: RCH=CH(CH2) n N·R1 →
cyclo-[NR1CH(CH2) n ]C·HR, R(CH2)2OOCH2C·HR → cyclo-[RCHOCH2] + RCH2CH2O·,
cyclo-[(CH2) n OOCHC· HR] → cyclo-[RCHOCH](CH2) n O·, cyclo-[(CH2) n OC·RO] →
RC(O)O(CH2) n − 1C·H2, and cyclo-[(CH2) n CHO·] → CH(O)(CH2) n − 1C·H2. The
activation en... hiện toàn bộ
Formation of the Ni–CrOx/MgO and Ni/MgO Catalysts for Carbon Dioxide Reforming of MethaneKinetics and Catalysis - - 2001
V. Yu. Bychkov, V. N. Korchak, O. V. Krylov, O. S. Morozova, T. I. Khomenko
Temperature-programmed reduction by hydrogen, temperature-programmed desorption
of O2, local X-ray spectral analysis, and scanning electron microscopy are used
to study redox processes occurring on the Ni–Cr2O3/MgO and Ni/MgO catalysts for
carbon dioxide reforming of methane. The reduction of Ni/MgO leads to the
formation of nickel clusters distributed over the surface of MgO. During the
reduction... hiện toàn bộ
A comparative study of Ir/Ga2O3, Pt/Ga2O3, and Ru/Ga2O3 catalysts in selective hydrogenation of crotonaldehydeKinetics and Catalysis - Tập 49 - Trang 574-580 - 2008
E. Gebauer-Henke, J. Farbotko, R. Touroude, J. Rynkowski
Catalytic performance of gallia-supported iridium catalysts in the reaction of
selective hydrogenation of crotonaldehyde in the gas phase was studied and
compared to that of platinum and ruthenium catalysts. The best catalytic
properties in terms of the selectivity to crotyl alcohol are shown by 5 wt %
Pt/α-Ga2O3 and 5 wt % Ir/α-Ga2O3 catalysts prepared from nonchlorine precursors:
Pt(acac)2 and I... hiện toàn bộ
Effect of water on the kinetics of the catalytic reaction between benzoic acid and anilineKinetics and Catalysis - Tập 48 - Trang 632-635 - 2007
L. Ya. Shteinberg, S. A. Kondratov, S. M. Shein, V. V. Marshalova
Water forming in benzanilide synthesis from benzoic acid and aniline catalyzed
by titanium tetrabutoxide does not influence the activity of the catalyst. The
role of mass transfer processes associated with water removal from the system is
revealed. The reversible deactivation of titanium tetrabutoxide by water occurs
in the absence of vigorous water boiling and distillation. The stability of
titan... hiện toàn bộ
Analysis and Simulation of the Dynamics of a Catalyzed Model Reaction: CO Oxidation on Zeolite Supported PalladiumKinetics and Catalysis - Tập 44 - Trang 183-197 - 2003
N. I. Jaeger, N. V. Peskov, M. M. Slinko
The particle size effect on the oscillatory behavior during CO oxidation over
zeolite-supported Pd catalysts is simulated with the help of a deterministic
point model and a stochastic mesoscopic model. The point model is developed on
the basis of the well-known Sales–Turner–Maple model, which is modified to
consider the slow processes of oxidation and reduction of the Pd bulk as well as
the effect... hiện toàn bộ