The morphology in nafion perfluorinated membrane products, as determined by wide‐ and small‐angle x‐ray studies

Wiley - Tập 19 Số 11 - Trang 1687-1704 - 1981
T. D. Gierke1, George. Munn1, Frank C. Wilson1
1E. I. du Pont de Nemours and Company, Plastic Products and Resins Department, Experimental Station, Wilmington, Delaware 19898

Tóm tắt

Abstract

The morphology of the ionomer resin from which Nafion perfluorinated membrane products are made was studied with wide‐angle and small‐angle x‐ray diffraction. A reflection observed in the small‐angle x‐ray scan from hydrolyzed polymer is attributed to ionic clustering. The effects of equiv wt, cation form, temperature, water content, and tensile drawing on this reflection were studied and are discussed.

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Tài liệu tham khảo

W. G. F.Grot G. E.Munn andP. N.Walmsley 141st Meeting of the Electrochemical Society Houston 1972 Abstract No. 154 [

10.1149/1.2404113

F. B.Leitz M. A.Accomazzo andS. A.Michalek 141st Meeting of the Electrochemical Society Houston 1972 Abstract No. 150 [

10.1149/1.2404113

L. J.NuttalandW. A.Titterington presented at the Conference on Electrolytic Production of Hydrogen London 1975.

10.1149/1.2128984

10.1021/jo00862a003

Olah G. A., 1978, Nouv. J. Chim., 2, 581

10.1055/s-1978-24945

Eisenberg A., 1977, Polymer Physics

10.1002/app.1977.070210401

T. D.Gierke 152nd Meeting of the Electrochemical Soc. Atlanta 1977 Abstract No. 438 [

1977, J. Electrochem. Soc., 124, 319C

10.1016/0032-3861(78)90176-3

10.1021/ja00492a008

10.1016/0032-3861(79)90103-4

10.1021/ac50012a031

C. J.Hora K. J.MauritzandA. J.Hopfinger 152nd Meeting of the Electrochemical Society Atlanta 1977 Abstract No. 439 [

1977, J. Electrochem. Soc., 124, 319C

10.1107/S0365110X60001138

10.1107/S0365110X65004681

Geil P. H., 1963, Polymer Single Crystals, 96

Wunderlich B., 1973, Macromolecular Physics

Wilson F. C., 1968, Polym. Prepr. Am. Chem. Soc. Div. Polym. Chem., 9, 505

10.1021/ma60033a007

10.1002/pol.1980.180180702

10.1002/polc.5070450110

10.1021/ma60014a006

T. D.Gierke S.Barenburg andR. R.Hebert to appear. It should be noted that the validity of such TEM results has been seriously questioned; see ref. 33.

H. W.Starkweather to appear.

Mauritz K., 1978, Polym. Prepr. Am. Chem. Soc. Div. Polym. Chem., 19, 336

T. D.Gierke 153rd Meeting of the Electrochemical Society Seattle 1978 Abstract No. 453 [

1978, J. Electrochem. Soc., 125, 163C

10.1021/ma60073a041

10.1021/ja00537a009

10.1021/j100477a008

A. J.Hopfinger private communication.

10.1021/ma50004a063

10.1002/pol.1981.180190101