Paracetamol oxidation from aqueous solutions by means of ozonation and H2O2/UV system

Water Research - Tập 37 Số 5 - Trang 993-1004 - 2003
Roberto Andreozzi1, V. Caprio1, Raffaele Marotta1, Davide Vogna2
1Dip. di Ingegneria Chimica, Facolta di Ingegneria, Universita degli Studi di Napoli Federico II, Piazzale V. Tecchio, 80-80125 Napoli, Italy.
2Universita degli Studi di Napoli “Federico II”, Facolta di Scienze, Dip. di Chimica Organica e Biochimica, Complesso Universitario M. S. Angelo, via Cinthia, 80126 Napoli, Italy

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Paxeus, 1996, Organic pollutants in the effluents of large wastewater treatment plants in Sweden, Water Res, 30, 1115, 10.1016/0043-1354(95)00278-2

Janssens, 1997, Micropollutants, Water Sci Technol, 35, 13, 10.2166/wst.1997.0349

Fromme, 2001, Polycyclic musk fragrances in different environmental compartments in Berlin (Germany), Water Res, 35, 121, 10.1016/S0043-1354(00)00233-5

Rodgers, 2000, Long-term temporal changes in the estrogenic compostion of treated sewage effluents and its biological effects on fish, Environ Sci Technol, 34, 1521, 10.1021/es991059c

Holm, 1995, Occurrence and distribution of pharmaceutical organic compounds in the groundwater downgradient of a landfill (Griendsted, Denmark), Environ Sci Technol, 29, 1415, 10.1021/es00005a039

Ternes, 1998, Occurrence of drugs in German sewage treatment plants and rivers, Water Res, 32, 3245, 10.1016/S0043-1354(98)00099-2

Daughton, 1999, Pharmaceuticals and personal care products in the environment, Environ Health Perspectives, 107, 907, 10.1289/ehp.99107s6907

Hirsch, 1999, Occurrence of antibiotics in the aquatic environment, Sci Total Environ, 225, 109, 10.1016/S0048-9697(98)00337-4

Buser, 1999, Occurrence and environmental behavior of the chiral pharmaceutical drug Ibuprofen in surface waters and in wastewater, Environ Science & Technology, 33, 2529, 10.1021/es981014w

Jorgensen, 2000, Drugs in the environment, Chemosphere, 40, 691, 10.1016/S0045-6535(99)00438-5

Buser HR, Poiger T, Muller MD Occurrence and fate of the pharmaceutical drug diclofenac in surface waters: rapid photodegradation in a lake. Environ Sci Technol 1998a;32(22): 3449–56.

Buser HR, Muller MD, Norbert T. Occurrence of the pharmaceutical drug clofibric acid and the herbicide mecoprop in various Swiss lakes and in the North Sea. Environ Sci Technol 1998b;32: 188–92.

Zuccato, 2000, Presence of therapeutic drugs in the environment, Lancet, 355, 1789, 10.1016/S0140-6736(00)02270-4

Halling-Sorensen, 1998, Occurrence, fate and effects of pharmaceutical substances in the environment- a review, Chemosphere, 36, 357, 10.1016/S0045-6535(97)00354-8

Burton K. An invader worse than a “B” movie. Endang. Species Bull 2000; XXV(5): 11–2.

Andreozzi R, Caprio V, Insola A, Marotta R. The oxidation of metol (N-methyl-p-aminophenol) in aqueous solution by UV/H2O2 photolysis. Water Res 2000a;34(2): 463–72.

Andreozzi R, Lo Casale MS, Marotta R, Pinto G, Pollio A. N-methyl-p-aminophenol (metol) ozonation in aqueous solution: kinetics, mechanism and toxicological characterization of ozonized samples. Water Res 2000b;34(18): 4419–29.

Lunar, 2000, Degradation of photographic developers by Fenton's reagent, Water Res, 34, 1791, 10.1016/S0043-1354(99)00339-5

Nicole, 1990, Use of UV radiation in water treatment, Water Res, 24, 157, 10.1016/0043-1354(90)90098-Q

Treadwell FP, Hall J. Analytical chemistry, vol. II (8th ed.) New York: John Wiley, 1935.

Andreozzi R, Insola A, Caprio V, D’Amore MG. Quinoline ozonation in aqueous solutions. Water Res 1992a;26(5): 639–44.

Bailey P S. Ozonation in organic chemistry, Vol. II. New York: Academic Press, 1982.

Karpel Vel Leitner, 1997, Mechanism of the reaction between hydroxyl radicals and glycolic, glyoxylic, acetic and oxalic acids in aqueous solution, Water Res, 31, 1383

Scheck, 1995, Degradation of phenol and salicylic acid by ultraviolet radiation/hydrogen peroxide/oxygen, Water Res, 29, 2346, 10.1016/0043-1354(95)00060-X

Andreozzi R, Insola A, Caprio V, D’Amore MG. Kinetics and mechanism of malonic acid ozonation in aqueous solution. Oxid Commun 1992b;15(2): 76–84.

Andreozzi, 1996, Measuring ozonation rate constants in gas–liquid reaction under the kinetic-diffusional transition regime, Chem Eng Commun, 143, 195, 10.1080/00986449608936441

Andreozzi, 1999, Ozonation of p-chlorophenol, J Hazard Mater, B69, 303, 10.1016/S0304-3894(99)00113-2

Reklaitis, 1983

Dastmalchi, 1995, Simultaneous determination of the pKa and octanol/water partition coefficient of acetaminophen, J. Sch. Pharm. , Med. Sci., 4, 7

Hunt, 1952, Decomposition of H2O2—quantum yields, tracer and fractionation effects, J Am Chem Soc, 74, 5999, 10.1021/ja01143a052

Buxton, 1988, Critical review of rate constants for reactions of hydrated electrons, hydrogen atoms and hydroxyl radicals (OH·/O−·) in aqueous solution, J Phys Chem Ref. Data, 17, 513, 10.1063/1.555805

Bielski, 1985, Reactivity of HO2/O2− radicals in aqueous solution, J Phys Chem Ref Data, 14, 1041, 10.1063/1.555739

Baxendale, 1957, Photolysis of hydrogen peroxide at high light intensities, Trans Faraday Soc, 53, 344, 10.1039/tf9575300344

Volman, 1959, The photochemical decomposition of hydrogen peroxide in aqueous solutios of allyl alcohol at 2537 A, J Am Chem Soc, 81, 4141, 10.1021/ja01525a004

Vogna, 2002, Advanced oxidation chemistry of paracetamol. UV/H2O2-induced hydroxylation/degradation pathways and 15N-aided inventory of nitrogenous breakdown products, J Org Chem, 67, 6143, 10.1021/jo025604v