Aggregation Effects on Electrochemical and Spectroelectrochemical Properties of [2,3,9,10,16,17,23,24-Octa(3,3-dimethyl-1-butynyl)phthalocyaninato]cobalt(II) ComplexBulletin of the Chemical Society of Japan - Tập 71 Số 5 - Trang 1039-1047 - 1998
Hiroaki Isago, Clifford C. Leznoff, Matthew F. Ryan, Robert A. Metcalfe, Rifka Davids, A. B. P. Lever
Abstract
The title complex, [Co(odmbpc)], which is a single isomer and is highly soluble in common organic solvents, has been prepared and investigated electrochemically and spectroelectrochemically in dichloromethane solutions. The cyclic voltammograms of this complex at a concentration of ca. 6 × 10−5 mol dm−3 exhibited two reversible reduction wav...... hiện toàn bộ
Orientation Effect of Side Chain Substituents in Aromatic Substitution. Induced Ortho NitrationBulletin of the Chemical Society of Japan - Tập 68 Số 4 - Trang 1155-1161 - 1995
Paolo Strazzolini, Giancarlo Verardo, Fausto Gorassini, Angelo G. Giumanini
Abstract
The presence of a free carboxyl or ester function on the α-carbon of toluene induces the nitration of the phenyl ring in the ortho position at or above the statistical value (chaperon effect), when pure HNO3 is used in CH2Cl2 solution. This is at variance with the results of classical nitration in H2SO4, where p-nitration predominates by far...... hiện toàn bộ
Acyliminium Cyclization of Several Chiral N-Alkenylsuccinimide DerivativesBulletin of the Chemical Society of Japan - Tập 63 Số 1 - Trang 287-289 - 1990
Jun Ohwada, Yoshinobu Inouye, Motoko Kimura, Hiroshi Kakisawa
Abstract
The acyliminium intermediate derived from (3R,4R)-N-(3-butenyl)-3,4-bis(benzyloxy)succinimide cyclized to give (8aS)- and (8aR)-hexahydro-3(2H)-indolidinone derivatives. On the other hand, those derived from N-3-hexenyl derivatives afforded (8aS)-hexahydro-3(2H)-indolidinone(s) exclusively. The geometry of the double bond reflected the stere...
Activation of Linear Alkanes by a Hydrido Triruthenium Cluster and Associated Skeletal RearrangementsBulletin of the Chemical Society of Japan - Tập 87 Số 4 - Trang 443-458 - 2014
Toshiro Takao, Hiroharu Suzuki
Abstract
We explored polyhydrido cluster reaction chemistry for over two decades, developing rational syntheses of di-, tri-, tetra-, and pentanuclear clusters of ruthenium. In our study of cluster chemistry, we found that triruthenium pentahydrido complex [{Cp*Ru(µ-H)}3(µ3-H)2] (1) (Cp*: η5-C5Me5) reacts with linear alkanes to exclusively afford a c...... hiện toàn bộ
Electronic Properties and π-π* Absorption Spectrum of 2-PyridoneBulletin of the Chemical Society of Japan - Tập 54 Số 9 - Trang 2802-2806 - 1981
Akira Fujimoto, Kōzō Inuzuka, Ryuichi Shiba
Abstract
The IR and U V absorption spectra as well as the Raman spectra of monomer and dimer of 2-pyridone were studied. The molecular weight of 2-pyridone in benzene and dimethyl sulfoxide was determined in order to examine the association. 2-Pyridone in nonpolar solvents shows two types of carbonyl stretching vibration bands due to the coexistence ...... hiện toàn bộ
EXAFS Studies of the Behavior of Rh6(CO)16 Supported on γ-Al2O3 SurfaceBulletin of the Chemical Society of Japan - Tập 59 Số 2 - Trang 647-648 - 1986
Kiyotaka Asakura, Yasuhiro Iwasawa, Haruo Kuroda
Abstract
The structural change of Rh6(CO)16 supported on γ-Al2O3 surface during a decarbonylation–recarbonylation cycle was studied by means of EXAFS (extended X-ray absorption fine structure) spectroscopy. Rh6(CO)16 cluster framework was found to be decomposed into Rh(CO)2(OAl(Remark: Graphics omitted.))2 after the reaction with a mixture of O2 and ...... hiện toàn bộ