The toxicology of chromium with respect to its chemical speciation: A review

Journal of Applied Toxicology - Tập 13 Số 3 - Trang 217-224 - 1993
Sidney Katz1, Harry Salem2
1Rutgers University, Camden, NJ 08102-1205, USA
2Chemical Research Development, and Engineering Centre, Toxicology Division, Aberdeen Proving Ground, MD 21010-5423, USA

Tóm tắt

Abstract

The properties of trivalent and hexavalent chromium are reviewed with respect to acute and chronic oral toxicity, dermal toxicity, systemic toxicity, toxicokinetics, cytotoxicity, genotoxicity and carcinogenicity. The hexavalent chromium compounds appear to be 10–100 times more toxic than the trivalent chromium compounds when both are administered by the oral route. Dermal irritancy and allergy are more frequently caused by contact with soluble hexavalent chromium compounds. The cytotoxicity of soluble and insoluble hexavalent chromium compounds to fibroblasts is 100‐1000 times greater than that demonstrated by trivalent chromium compounds. In short‐term tests, the hexavalent chromium compounds demonstrated genotoxic effects four times more frequently than did the trivalent chromium compounds. Carcinogenicity appears to be associated with the inhalation of the less soluble/insoluble hexavalent chromium compounds. The toxicology of chromium does not reside with the elemental form. It varies greatly among a wide variety of very different chromium compounds. Oxidation state and solubility are particularly important factors in considering the toxicity of chromium with respect to its chemical speciation.

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Tài liệu tham khảo

10.1002/tcm.1770050507

Levy L. S., 1936, Investigation of the potential carcinogenicity of a range of chromium containing materials on rat lung, Br. J. Ind. Med., 43, 243

Samitz M. H., 1955, Some dermatologic aspects of the chromate problem, Arch. Ind. Health, 11, 361

Popper H. H., 1991, Progress in Histo‐Cytochemistry as a Tool in Environmental Toxicology, 220

10.1292/jvms.54.281

10.1080/02772248909357424

10.1080/02772248809357274

10.1080/02772248909357455

10.1152/physrev.1969.49.2.163

10.1016/0048-9697(89)90196-4

Schroeder H. A., 1963, Effect of chromium, cadmium and lead on the growth and survival of rats, J. Nutr., 80, 39

Emsley J., 1989, The Elements, 50

10.1016/0039-9140(76)80040-9

10.1021/ja01326a010

Rieman W., 1951, J. Am. Chem. Soc., 325

Weast R. C., 1970, CRC Handbook of Chemistry and Physics

Dean J. A., 1979, Lang's Handbook of Chemistry

Dean J. A., 1985, Lang's Handbook of Chemistry

Linke W. F., 1958, Solubilities of Inorganic and Metal‐Organic Compounds

10.1093/carcin/12.4.551

Registry of Toxic Effects of Chemical Substances, 1986, US Department of Health and Human Services, Public Health Service, Centers for Disease Control

Samitz M. H., 1964, A current review of the chromate problem, Dermatol. Dig., 3, 18

Samitz M. H., 1962, Studies on the prevention of the injurious effects of chromates in industry, Ind. Med. Surg., 31, 427

MacKenzie R. D., 1958, Chronic toxicity studies. II. Hexavalent and trivalent chromium administered in drinking water to rats, Arch. Ind. Health, 18, 232

10.1093/jn/86.1.51

10.1016/S0015-6264(75)80298-7

10.1080/00039896.1962.10663312

10.1001/archderm.1961.01580150050009

10.1038/jid.1963.83

10.1001/archderm.1964.01600010010003

10.1001/archderm.1965.01600090041007

Fregert S., 1966, Allergy to chromium, nickel and cobalt, Arch. Dermatol Venerol., 46, 144

10.1001/archderm.93.1.34

Samitz M. H., 1966, Patch test reactions to hexavalent and trivalent chromium compounds, Arch. Dermatol., 94, 304, 10.1001/archderm.1966.01600270054010

Valer M., 1971, Investivation concerning the sensitizing effect of trivalent chromium salts, Berufs‐Dermatosen, 6, 302

10.1177/096032719101000315

10.1177/096032719101000207

10.1159/000181540

10.1093/jat/12.3.162

10.1007/BF00398817

10.3109/15563658209025729

10.1016/0041-008X(81)90111-3

10.1016/0300-483X(77)90023-3

10.1016/0041-008X(86)90384-4

10.1007/BF01973713

10.1093/annhyg/27.3.315

10.1016/0048-9697(89)90193-9

10.1152/ajplegacy.1965.209.4.731

Mertz W., 1965, Biological activity and fate of trace quantities of intravenous chromium(III) in the rat, Am. J. Physiol., 209, 614, 10.1152/ajplegacy.1965.209.3.489

10.1248/bpb1978.3.17

10.2486/indhealth.21.25

10.1172/JCI102403

10.3891/acta.chem.scand.13-0456

10.1007/BF02992700

Anhgileri L. J., 1965, Fate of injected homologour 51Cr labeled sero‐albumin in rats, Nuc. Med., 9, 364

Lim T. H., 1983, Kinetics of trace element chromium(III) in the human body, Am. J. Physiol., 244, 445

Biedermann K. A., 1990, Role of valence state and solubility of chromium compounds on induction of cytotoxicity, mutagenesis, and anchorage independence in diploid human fibroblasts, Cancer Res., 50, 7835

10.1007/BF01973630

10.1093/carcin/12.10.1811

10.1016/0272-0590(88)90322-3

10.1016/0022-1759(91)90217-4

10.1016/0022-1759(92)90257-T

10.1016/0925-4439(92)90046-P

10.1016/0165-1110(90)90007-X

Baetjer A. M., 1950, Pulmonary carcinoma in chromate workers. I. A review of the literature and report of cases, Arch. Ind. Hyg. Occup., 2, 487

Baetjer A. M., 1950, Pulmonary carcinoma in chromate workers. II. Incidence on basis of hospital records, Arch. Ind. Hyg. Occup. Med., 2, 505

Bidstrup P. L., 1951, Carcinoma of the lung in chromate workers, Br. J. Ind. Med., 8, 302

Bidstrup P. L., 1956, Carcinoma in the lung of workmen in the bichromate‐producing industry in Great Britain, Br. J. Ind. Med., 13, 260

10.1055/s-0028-1122461

10.1093/ije/8.4.365

10.1016/0013-9351(75)90072-9

10.1016/0013-9351(75)90079-1

10.1007/BF00406930

10.5271/sjweh.2413

Satoh K., 1981, Epidemiological study of workers engaged in the manufacture of chromium compounds, J. Occup. Med., 23, 835

U.Glaser D.HochrainerandH.Oldiges Investigation of the lung carcinogenic potentials of sodium dichromate and Cr VI/III oxide aerosols in Wistar rats. First European Meeting on Environmental Hygiene pp.111–116(1988).

Hueper W. C., 1961, Environmental carcinogens and cancers, Cancer Res., 21, 824

10.1080/00039896.1962.10663311

10.1093/jn/83.3.239

10.1038/bjc.1975.201

Laskin S., 1970, Inhalation Carcinogenesis

Nettesheim P., 1971, Effect of calcium chromate dust, influenza virus, and 100 R whole body X‐radiation on lung tumor incidence in mice, J. Natl. Cancer Inst., 47, 1129

Laskin S., 1972, Research in Environmental Sciences, 92

Sixth Annual Report on Carcinogens Summary 1991 pp.52–53. US Department of Health and Human Services Public Health Service Washington DC (1991).