Sub‐10‐fs Timing for Ultrafast Electron Diffraction with THz‐Driven Streak Camera

Laser and Photonics Reviews - Tập 15 Số 2 - 2021
Junho Shin1, Hyun Woo Kim1, In Hyung Baek1, Seong Hee Park1, Hyeon Sang Bark1, Key Young Oang1, Kyu‐Ha Jang1, Kitae Lee1, Fabıan Rotermund2, Young Uk Jeong1, Jungwon Kim2
1Radiation Center for Ultrafast Science, Korea Atomic Energy Research Institute (KAERI), Daejeon, 34057 Republic of Korea
2Korea Advanced Institute of Science and Technology (KAIST), Daejeon 34141, Republic of Korea

Tóm tắt

AbstractUltrafast electron diffraction (UED) has evolved to be a powerful tool for the study of structural dynamics with subpicosecond temporal resolution and subatomic spatial resolution. Recently, there have been intense research efforts toward femtosecond timing jitter and stability for improving the temporal resolution of UEDs, however, so far there has been no work showing long‐term (e.g., >1 h) stable timing for MeV‐level UED systems. In this article, a comprehensive timing synchronization method, based on optical‐radiofrequency synchronization and THz streaking, is demonstrated to maintain sub‐10‐fs long‐term timing stability for radiofrequency‐gun‐based MeV‐level UED, which results in 5.5 fs root‐mean‐square timing drift maintained over 4600 s. With high electron energy and low timing drift, the demonstrated capability is an important step toward studying ultrafast phenomena in samples with low scattering power, such as volatile gases and 2D materials.

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Tập 15 Số 2

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