Reactions of 1-vinylbenzimidazole-2-thione with alcohols and phenol

Chemistry of Heterocyclic Compounds - Tập 20 - Trang 656-658 - 1984
N. D. Abramova1, G. G. Skvortsova1, B. V. Trzhtsinskaya1
1Irkutsk Institute of Organic Chemistry, Siberian Branch, Academy of Sciences of the USSR, Irkutsk

Tóm tắt

1-(α-Alkoxyethyl)- and 1-(α-phenoxyethyl)benzimidazole-2-thiones were obtained in the reaction of 1-vinylbenzimidazole-2-thione with alcohols and phenol in the presence of gaseous hydrogen chloride. It was established that partial hydrolysis of the 1-(α-alkoxyethyl)benzimidazole-2-thiones to benzimidazole-2-thione with subsequent alkylation with excess alcohol at the exocyclic sulfur atom occurs under the conditions of the investigated reaction. A convenient method for the alkylation of thiones was proposed, and a number of 2-alkylthiobenzimidazoles were synthesized.

Tài liệu tham khảo

N. D. Abramova, G. G. Skvortsova, B. V. Trzhtsinskaya, and M. V. Sigalov, Khim. Geterotsikl. Soedin., No. 12, 1674 (1975). M. L. Martin, F. Lefevre, D. Lapeyre, and G. Martin, J. Org. Magn. Reson., 1, 19 (1969). G. G. Skvortsova, E. S. Domnina, N. P. Glaskova, N. N. Chipanina, and N. I. Shergina, Zh. Obshch. Khim., 41., 623 (1971). K. Futaki, J. Pharm. Soc. Japan, 74, 1365 (1954); Chem. Abstr., 49, 15876 (1955).