Excited state properties of chlorophyll f in organic solvents at ambient and cryogenic temperatures

Photosynthesis Research - Tập 121 - Trang 25-34 - 2014
Dariusz M. Niedzwiedzki1, Haijun Liu1,2, Min Chen3, Robert E. Blankenship1,2,4
1Photosynthetic Antenna Research Center, Washington University in St. Louis, St. Louis, USA
2Department of Biology, Washington University in St. Louis, St. Louis, USA
3School of Biological Sciences, University of Sydney, Sydney, Australia
4Department of Chemistry, Washington University in St. Louis, St. Louis, USA

Tóm tắt

Chlorophyll f is a photosynthetic pigment that was discovered in 2010. In this study, we present investigations on spectral and dynamic characteristics of singlet-excited and triplet states of Chl f with the application of ultrafast time-resolved absorption and fluorescence spectroscopies. The pigment was studied at room temperature in two organic solvents: pyridine and diethyl ether that have different characters of coordination of the chlorophyll magnesium (Mg) atom (hexa- and penta-coordination, respectively). Cryogenic measurements (77 K) were performed in 2-methyltetrahydrofuran (hexa-coordination). The singlet-excited state lifetime was measured to be 5.6 ns at room temperature regardless of Mg coordination and 8.1 ns at 77 K. The fluorescence quantum yield of Chl f was also determined in pyridine to be 0.16. The triplet state lifetime was studied in detail in pyridine at room temperature, and the inherent lifetime was estimated to ~150 μs. Selective measurements at 77 K demonstrated that the metastability of the triplet state greatly enhances, and its lifetime increases by a factor of more than three.

Tài liệu tham khảo

Brody SS, Rabinowitch E (1957) Excitation lifetime of photosynthetic pigments in vitro and in vivo. Science 125:555 Chen M, Blankenship RE (2011) Expanding the solar spectrum used by photosynthesis. Trends Plant Sci 16:427–431 Chen M, Schliep M, Willows RD, Cai ZL, Neilan BA, Scheer H (2010) A red-shifted chlorophyll. Science 329:1318–1319 Chen M, Li YQ, Birch D, Willows RD (2012) A cyanobacterium that contains chlorophyll f—a red-absorbing photopigment. FEBS Lett 586:3249–3254 Connolly JS, Janzen AF, Samuel EB (1982) Fluorescence lifetimes of chlorophyll a—solvent, concentration and oxygen dependence. Photochem Photobiol 36:559–563 Fujimori E, Livingston R (1957) Interactions of chlorophyll in its triplet state with oxygen, carotene, etc. Nature 180:1036–1038 Gouterman M (1959) Study of the effects of substitution on the absorption spectra of porphyrin. J Chem Phys 30:1139–1161 Gouterman M (1961) Spectra of porphyrins. J Mol Spectrosc 6:138–163 Gouterman M (1978) Optical spectra and electronic structure of porphyrins and related rings. In: Dolphin D (ed) Physical chemistry: Part A. Academic Press, New York, pp 1–166 Hindman JC, Kugel R, Svirmickas A, Katz JJ (1978) Stimulated fluorescence and fluorescence quenching in chlorophyll a and bacteriochlorophyll a. Chem Phys Lett 53:197–200 Latimer P, Bannister TT, Rabinowitch E (1956) Quantum yields of fluorescence of plant pigments. Science 124:585–586 Li YQ, Scales N, Blankenship RE, Willows RD, Chen M (2012) Extinction coefficient for red-shifted chlorophylls: chlorophyll d and chlorophyll f. Biochim Biophys Acta 1817:1292–1298 Li Y, Cai ZL, Chen M (2013) Spectroscopic properties of chlorophyll f. J Phys Chem B 117:11309–11317 Manning WM, Strain HH (1943) Chlorophyll d, a green pigment of red algae. J Biol Chem 151:1–19 Miyashita H, Ikemoto H, Kurano N, Adachi K, Chihara M, Miyachi S (1996) Chlorophyll d as a major pigment. Nature 383:402 Natarajan LV, Ricker JE, Blankenship RE, Chang R (1984) Solvent influences on the singlet quenching of chlorophyll a by 2,5-dimethyl-para-benzoquinone. Photochem Photobiol 39:301–306 Niedzwiedzki DM, Blankenship RE (2010) Singlet and triplet excited state properties of natural chlorophylls and bacteriochlorophylls. Photosynth Res 106:227–238 Niedzwiedzki DM, Fuciman M, Frank HA, Blankenship RE (2011) Energy transfer in an LH4-like light harvesting complex from the aerobic purple photosynthetic bacterium Roseobacter denitrificans. Biochim Biophys Acta 1807:518–528 Pelletier PJ, Caventou JB (1818) Sur la matière verte des feuilles. Ann Chim Phys 9:194–196 Strain HH (1958) Chloroplast pigments and chromatographic analysis. Pennsylvania State University, University Park van Stokkum IH, Larsen DS, van Grondelle R (2004) Global and target analysis of time-resolved spectra. Biochim Biophys Acta 1657:82–104 Weiss C (1972) π-electron structure and absorption spectra of chlorophylls in solution. J Mol Spectrosc 44:37–80 Williams ATR, Winfield SA, Miller JN (1983) Relative fluorescence quantum yields using a computer-controlled luminescence spectrometer. Analyst 108:1067–1071 Yamijala SRKCS, Periyasamy G, Pati SK (2011) Computational studies on structural and excited-state properties of modified chlorophyll f with various axial ligands. J Phys Chem A 115:12298–12306 Zapata M, Garrido J, Jeffrey SW (2006) Chlorophyll c pigments: current status. In: Grimm B, Porra RJ, Rudiger W, Scheer H (eds) Chlorophylls and bacteriochlorophylls: biochemistry, biophysics, function and applications (advances in photosynthesis and respiration). Springer, New York, pp 39–53