Excitation Spectra of Circular, Few-Electron Quantum Dots

American Association for the Advancement of Science (AAAS) - Tập 278 Số 5344 - Trang 1788-1792 - 1997
Leo P. Kouwenhoven1,2,3, Tjerk H. Oosterkamp1,2,3, M. W. S. Danoesastro1,2,3, Mikio Eto1,2,3, D. G. Austing1,2,3,4, Takashi Honda1,2,3,4, Seigo Tarucha1,2,3,4
1D. G. Austing, T. Honda, S. Tarucha, NTT Basic Research Laboratories, 3-1, Morinosoto Wakamiya, Atsugi-shi, Kanagawa 243-01, Japan.
2L. P. Kouwenhoven, T. H. Oosterkamp, M. W. S. Danoesastro, Department of Applied Physics and Delft Institute of MicroElectronics and Submicrontechnology, Delft University of Technology, Post Office Box 5046, 2600 GA Delft, Netherlands.
3M. Eto, Department of Physics, Faculty of Science and Technology, Keio University, 3-14-1 Hiyoshi, Kohoku-ku, Yokohama 223, Japan.
4Nippon Telegraph & Telephone

Tóm tắt

Studies of the ground and excited states in semiconductor quantum dots containing 1 to 12 electrons showed that the quantum numbers of the states in the excitation spectra can be identified and compared with exact calculations. A magnetic field induces transitions between the ground and excited states. These transitions were analyzed in terms of crossings between single-particle states, singlet-triplet transitions, spin polarization, and Hund's rule. These impurity-free quantum dots allow “atomic physics” experiments to be performed in magnetic field regimes not accessible for atoms.

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Tài liệu tham khảo

Ashoori R. C., Nature 379, 413 (1996).

For a review see L. P. Kouwenhoven et al. Proceedings of the Advanced Study Institute on Mesoscopic Electron Transport Curaçao 25 June to 5 July 1996 (Series E Kluwer Dordrecht Netherlands in press). Also available on the World Wide Web at .

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M. Alonso and E. J. Finn Quantum and Statistical Physics (Addison-Wesley Reading MA 1968).

10.1103/PhysRevLett.78.1544

Figure 2 actually reproduces in large detail in four different samples implying that the structure in the density of states in the leads is not originating from a random impurity potential but probably from the lateral confinement potential of the pillar.

The sign of V sd is such that electrons first tunnel through the thicker barrier. In this situation only the excited states above the ground-state electrochemical potential are observed. For equal tunnel barriers tunneling out of the dot from excited states below the ground-state electrochemical potential can also be measured; see (2). Note that for a thick enough entrance barrier we can assume relaxation to the ground state between tunneling out and tunneling into the dot of the next electron.

See for example J. J. Palacios L. Martin-Moreno G. Chiappe E. Louis C. Tejedor Phys. Rev. B 50 5760 (1994); for more references see the review by

Johnson N. F., J. Phys. Condens. Matter 7, 965 (1995) .

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; C. G. Darwin Proc. Cambridge Philos. Soc. 27 86 (1930).

We believe that the smaller slopes in the experimental data of Fig. 5 for B > ∼7 T are due to a changing confinement potential because screening from the leads is modified by the formation of Landau levels in the leads. This is also reflected in the changing stripe width at high B.

Thurner G., Herold H., Ruder H., Schlicht G., Wunner G., Phys. Lett. 89A, 133 (1982).

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Schmidt T., et al., Phys. Rev. B 51, 5570 (1995).

For details of the calculation see

Eto M., Jpn. J. Appl. Phys. 36, 3924 (1997);

. In the numerically exact calculations every electron is assumed to occupy one of the lowest 15 single-particle states at B = 0. The strength of the Coulomb interaction is fixed such that e 2 / ε ℏ︀/m*ωo = ℏ︀ω o (ε is the permittivity). (Interactions between electrons in the dot and in the leads are neglected.) The calculated results indicate that the many-body states consist of one main configuration [two main configurations for N = 3 and ( S M ) = (½ 2)] and several small contributions from other configurations. The depicted configurations in Fig. 3 overlap by ∼70% or more with the many-body ground states (the spin-polarized states overlap by more than 95%).

For a theoretical analyses of the N = 2 excitation spectrum see for example

Pfannkuche D., Gerhardts R. R., Maksym P. A., Gudmundsson V., Physica B 189, 6 (1993).

Also for N ∼ 100 quantum dots the excitation spectra of N and N + 1 can be strongly correlated as observed recently by D. R. Stewart et al. [

10.1126/science.278.5344.1784

We thank R. J. van der Hage J. Janssen Y. Kervennic J. E. Mooij S. K. Nair L. L. Sohn Y. Tokura and T. Uesugi for help and discussions. Supported by the Dutch Foundation for Fundamental Research on Matter. L.P.K. was supported by the Royal Netherlands Academy of Arts and Sciences.