Effect of polyethylene addition to coal on hydrogasification enhancement

Journal of Material Cycles and Waste Management - Tập 16 - Trang 151-155 - 2013
Hajime Yasuda1, Osamu Yamada1, Mamoru Kaiho1, Hideki Nakagome2
1National Institute of Advanced Industrial Science and Technology (AIST), Tsukuba, Japan
2Graduate School and Faculty of Engineering, Chiba University, Chiba, Japan

Tóm tắt

Hydrogasification of a coal/polyethylene mixture was carried out using a low concentration of polyethylene in the samples with the aim of industrial application. Coal/polyethylene mixtures in the ratio of 90:10 and 75:25 were used in this study. A hydrogasification experiment was conducted using a unique batch reactor at 1073 K under a 7.1 MPa hydrogen atmosphere. The reaction time varied from 1 to 80 s. The results revealed a methane yield from the mixtures that was noticeably greater than the values calculated from experimental results obtained from coal and polyethylene respectively, assuming no mutual influences. A significant synergistic effect was observed even when the polyethylene content was as low as 10 %. It is suggested that there might be an advantage in hydrogasification processes if waste plastics are mixed with coal, such content being practically assumed.

Tài liệu tham khảo

Noguchi F, Maruyama H, Tsuru Y (2000) Coal hydrogasification process for the production of SNG and chemicals. Annu Int Pittsburgh Coal Conf 17:1375–1384 Asaoka Y, Azuma T, Yamauchi S, Kawamoto M, Tanaka T, Maruyama H (2000) Development of coal hydrogasification technology 3. Simulation incorporated the hydro-pyrolysis model into computational fluid dynamics. Annu Int Pittsburgh Coal Conf 17:523–539 Itoh K, Noguchi F, Katsukura K, Maruyama H (1999) Development of Coal Hydrogasification Technology. Prospects for Coal Science in the 21st Century (10th ICCS) 1: 599–602 Lackner KS, Yegulalp T (2005) Thermodynamic foundation of the zero emission concept. Miner Metall Process 22:161–167 Zhang A, Kaiho M, Yasuda H, Zabat M, Nakano K, Yamada O (2005) Fundamental studies on hydrogasification of Taiheiyo coal. Energy 30:2243–2250 Yasuda H, Yamada O, Zhang A, Nakano K, Kaiho M (2004) Hydrogasification of coal and polyethylene mixture. Fuel 83:2251–2254 Lee SH, Lee JG, Kim JH, Choi YC (2006) Hydrogasification characteristics of bituminous coals in an entrained-flow hydrogasifier. Fuel 85:803–806 Perdikaris N, Panopoulos KD, Fryda L, Kakaras E (2009) Design and optimization of carbon-free power generation based on coal hydrogasification integrated with SOFC. Fuel 88:1365–1375 Romano MC, Lozza GG (2010) Long-term coal gasification-based power plants with near-zero emissions. Part A: Zecomix cycle. Int J Greenh Gas Con 4:459–468 Romano MC, Lozza GG (2010) Long-term coal gasification-based power with near-zero emissions. Part B: Zecomag and oxy-fuel IGCC cycles. Int J Greenh Gas Con 4:469–477 Zhang AH, Kaiho M, Yasuda H, Zabat M, Yamada O (2002) Investigation on initial stage of rapid pyrolysis at high pressure using Taiheiyo coal in dense phase. Fuel 81:1189–1197 Yasuda H, Kamo T, Adachi M, Sajima S, Nakagome H (2010) Rapid hydropyrolysis of model compounds for epoxy resin oligomers and biomass tar. J Mater Cycles Waste Manag 12:123–127