Rate constants for the gas‐phase reactions of O3 with a series of monoterpenes and related compounds at 296 ± 2 K

International Journal of Chemical Kinetics - Tập 22 Số 8 - Trang 871-887 - 1990
Roger Atkinson1, David Hasegawa1, Sara M. Aschmann1
1Statewide Air Pollution Research Center, University of California, Riverside, California 92521

Tóm tắt

Abstract

Rate constants for the gas‐phase reactions of O3 with a series of monoterpenes and related compounds have been determined at 296 ± 2 K and 740 torr total pressure of air or O2 using a combination of absolute and relative rate techniques. Good agreement between the absolute and relative rate data was observed, and the rate constants obtained (in units of 10−17 cm3 molecule−1 s−1) were: α‐pinene, 8.7; β‐pinene, 1.5; Δ3‐carene, 3.8; 2‐carene, 24; sabinene, 8.8; d‐limonene, 21; γ‐terpinene, 14; terpinolene, 140; α‐phellandrene, 190; α‐terpinene, 870; myrcene, 49; trans‐ocimene, 56; p‐cymene, <0.005; and 1,8‐cineole, <0.015. While these rate constants for α‐ and β‐pinene and sabinene are in good agreement with recent absolute and relative rate determinations, those for the other monoterpenes are generally lower than the literature data by factors of ca. 2–10. The measured rate constants for the monoterpenes are reasonably consistent with predictions based upon the number and positions of the substituent groups around the 〉CC〈 bond(s).

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Tài liệu tham khảo

10.1029/RG017i005p00937

P. R.Zimmerman Tampa Bay area photochemical oxidant study. Final Report Appendix C. Determination of emission rates of hydrocarbons from indigenous species of vegetation in the Tampa/St. Petersburg Florida area. EPA 904/9‐77‐028 U.S. Environmental Protection Agency Atlanta Georgia February1979.

10.1104/pp.65.5.797

10.1086/botanicalgazette.143.3.2474826

10.1029/JC088iC15p10667

10.1029/JC088iC15p10679

10.1016/0004-6981(85)90131-3

10.1021/es00134a011

10.1029/JD093iD02p01407

10.1016/0045-6535(88)90223-8

10.1029/JD093iD04p03751

10.1016/0004-6981(88)90497-0

S.Juuti J.Arey andR.Atkinson J. Geophys. Res. in press (1990).

J.Arey A. M.Winer R.Atkinson S. M.Aschmann W. D.Long C. L.Morrison andD. M.Olszyk J. Geophys. Res. to be submitted for publication(1990).

10.1029/GL005i008p00679

10.1016/0004-6981(87)90108-9

10.1021/j100555a024

10.1021/es00106a004

10.1002/kin.550180303

R.Atkinson S. M.Aschmann andJ.Arey Atmos. Environ. in press.

Atkinson R., 1989, J. Phys. Chem. Ref. Data, 1

10.1021/es00123a016

10.1021/es00132a009

10.1021/j100323a028

10.1021/j100340a015

10.1021/ba-1972-0113.ch008

10.1080/00139307409437404

Grimsrud E. P., 1975, Int. J. Chem. Kinet., Symp., 1, 183

10.1016/0004-6981(82)90187-1

10.1021/cr00063a002

10.1007/BF00048331

10.1002/kin.550140103

10.1021/j100560a002

10.1021/ja00458a033

10.1002/kin.550101003

10.1016/0009-2614(80)80326-5

10.1021/ja00403a031

10.1021/j100288a035

10.1021/j100288a036

10.1002/kin.550060509

10.1021/j100614a004

Adams R. P., 1989, Identification of Essential Oils by Ion Trap Mass Spectrometry

10.1016/0960-1686(90)90438-S

10.1021/j150664a061