Ultrathin Graphitic C3N4 Nanosheets/Graphene Composites: Efficient Organic Electrocatalyst for Oxygen Evolution Reaction

Wiley - Tập 7 Số 8 - Trang 2125-2130 - 2014
Jingqi Tian1,2, Qian Liu2, Abdullah M. Asiri3, Khalid A. Alamry3, Xuping Sun3,2
1Graduate School of the Chinese Academy of Sciences, Beijing 100039, China
2State Key Laboratory of Electroanalytical Chemistry, Changchun Institute of Applied Chemistry, Changchun, 130022 Jilin, China
3Chemistry Department & Center of Excellence for Advanced Materials Research, King Abdulaziz University, Jeddah 21589, Saudi Arabia

Tóm tắt

AbstractGraphitic C3N4 (g‐C3N4) is used as a low‐cost organic oxygen evolution reaction (OER) electrocatalyst. The integration of ultrathin g‐C3N4 nanosheets with graphene leads to g‐C3N4/graphene composites with high OER activity and good durability. X‐ray photoelectron spectroscopy (XPS) studies suggest that the OER activity results from pyridinic‐N‐related active sites. This catalyst provides an alternative to OER catalysts based on transition metals.

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