Synthesis of monodisperse poly(divinylbenzene) microspheres

Wiley - Tập 31 Số 13 - Trang 3257-3263 - 1993
Kai Li1, Harald D. H. Stöver1
1Department of Chemistry, McMaster University, Hamilton, Ontario, Canada L8S 4M1

Tóm tắt

Abstract

Highly crosslinked monodisperse poly(divinylbenzene) microspheres were produced by precipitation polymerization with acetonitrile as solvent. The radical initiators AIBN, BPO, and ADVN were used. The process does not require stabilizers of any type, and produces monodisperse particles with diameters between 2 and 5 μm, depending on the conditions. These microspheres do not swell or dissolve in any common solvent, and have clean, stabilizer‐free surfaces. The particle formation and growth mechanism is proposed to resemble that of dispersion polymerization, except that the particles are stabilized against coagulation by their rigid, crosslinked surfaces rather than by added stabilizers. Spherical particles were formed only at effective crosslinker/monomer or divinyl/monovinyl ratios larger than 1 : 2. © 1993 John Wiley & Sons, Inc.

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Tài liệu tham khảo

10.1021/bk-1981-0165

10.1016/0001-8686(80)87003-5

10.1002/polc.5070720125

10.1002/pol.1985.130230209

10.1007/978-94-009-3685-0_13

10.1002/pola.1986.080241126

10.1002/pola.1990.080280921

Li K., 1992, Preparation and Characterization of Highly Crosslinked Polymer Particles from Commercial Divinylbenzene

M.Hattori E. D.Sudol andM. S.El‐Aasser Highly Crosslinked Polymer Particles by Dispersion Polymerization 34th IUPAC International Symposium on Macromolecules Prague July 13–18 1992.

10.1002/pola.1993.080311007

10.1002/pol.1977.170150912

10.1002/pola.1990.080280911

10.1002/apmc.1992.051950112

10.1002/pola.1990.080280722

10.1007/BF00665495

10.1002/pola.1992.080300726

10.1002/pola.1992.080300706

4‐Methylstyrene without any divinylbenzene can be polymerized to form spherical particles but requires polymeric stabilizers such as polyvinylpyrrolidone. This falls in the area of dispersion polymerization.

Brandrup J., 1975, Polymer Handbook

Riddick J. A., 1986, Organic Solvents—Physical Properties and Methods of Purification