Synthesis and hydrodynamic and molecular characteristics of N-methacryloylglucosamine N-vinylformamide copolymers

Pleiades Publishing Ltd - Tập 80 - Trang 777-782 - 2007
G. M. Pavlov1,2, E. V. Korneeva1,3, N. P. Ivanova1,2, O. A. Pavlova1,2, E. F. Panarin1,2
1Institute of Macromolecular Compounds, Russian Academy of Sciences, St. Petersburg, Russia
2Fock Institute of Physics, St. Petersburg State University, St. Petersburg, Russia
3Fock Institute of Physics, St.-Petersburg State University, St.-Petersburg, Russia

Tóm tắt

Random 50: 50 N-methacryloylglucosamine-N-vinylformamide copolymers were synthesized, and their hydrodynamic and molecular characteristics were examined. For the copolymers with the molecular weight 70 < M × 10−3 g mol−1 < 570 in 0.2 M NaCl, the Kuhn-Mark-Houwink-Sakurada equations were obtained, which relate the intrinsic viscosity and the translational diffusion and centrifugal sedimentation coefficients, on the one hand, to the molecular weight, on the other. The length of the statistical segment of the copolymer chains was estimated.

Tài liệu tham khảo

Panarin, E.F. and Ivanova, N.P., Zh. Prikl. Khim., 2005, vol. 78, no. 8, pp. 1340–1343. Pavlov, G.M., Korneeva, E.V., Mikhailova, N.A., et al., Vysokomol. Soedin., Ser. A, 1993, vol. 35, no. 10, pp. 1646–1651. Pavlov, G.M., Ivanova, N.P., Korneeva, E.V., et al., Carbohydrate Chem., 1996, vol. 15, no. 4, pp. 417–433. Pavlov, G.M., Korneeva, E.V., Ebel, C., et al., Vysokomol. Soedin., Ser. A, 2004, vol. 46, no. 10, pp. 1732–1737. Tsvetkov, V.N., Eskin, S.Ya., and Frenkel, S.Ya., Struktura makromolekul v rastvorakh (Structure of Macromolecules in Solutions), Moscow: Nauka, 1964. Kratky, O., Leopold, H., and Stabinger, H., Meth. Enzymol., 1973, vol. 27, pp. 98–110. Schuck, P., Biophys. J., 2000, vol. 78, pp. 1606–1619. Pavlov, G.M. and Frenkel, S.Ya., Vysokomol. Soedin., Ser. B, 1982, vol. 24, no. 3, pp. 173–180. Skazka, V.S., Sedimentatsionno-diffuzionnyi analiz polimerov v rastvore (Sedimentation and Diffusion Analysis of Polymers in Solution), Leningrad: Leningr. Gos. Univ., 1985. Tsvetkov, V.N., Zhestkotsepnye polimernye molekuly (Rigid-Chain Polymer Molecules), Leningrad: Nauka, 1986. Pavlov, G.M. and Frenkel, S.Ya., Vysokomol. Soedin., Ser. B, 1986, vol. 28, no. 5, pp. 353–357. Pavlov, G.M., Eur. Biophys. J., 1997, vol. 25, nos. 5/6, pp. 385–397. Budtov, V.P., Fizicheskaya khimiya rastvorov polimerov (Physical Chemistry of Polymer Solutions), St. Petersburg: Khimiya, 1992. Pavlov, G.M., Prog. Colloid. Polym. Sci., 2002, vol. 119, pp. 149–157. Ptitsyn, O.B. and Eizner, Yu.E., Zh. Tekh. Fiz., 1959, vol. 29, no. 9, pp. 1105–1112. Gray, G., Bloomfield, V., and Hearst, J., J. Chem. Phys., 1967, vol. 46, pp. 1493–1500. Pavlov, G.M., Panarin, E.F., Korneeva, E.V., et al., Vysokomol. Soedin., Ser. A, 1990, vol. 32, no. 6, pp. 1190–1192. Pavlov, G.M., Vysokomol. Soedin., Ser. A, 2004, vol. 46, no. 10, pp. 1872–1878.