Photofixation of atmospheric nitrogen to ammonia with a novel ternary metal sulfide catalyst under visible light

RSC Advances - Tập 6 Số 55 - Trang 49862-49867
Yuhui Cao1,2,3,4, Shaozheng Hu1,2,3,4, Fayun Li1,2,3,4, Zhiping Fan1,2,3,4, Jin Bai1,2,3,4, Guang Lü1,2,3,4, Qiong Wang1,2,3,4
1China
2College of Chemistry, Chemical Engineering and Environmental Engineering, Liaoning Shihua University, Fushun, China
3Fushun
4Liaoning ShiHua University

Tóm tắt

The NH4+ generation rate over ternary metal sulfide catalysts are linearly related to the sulfur vacancies concentration, confirming the photofixation capacity of N2 over ternary metal sulfide are dependent on the amount of sulfur vacancies.

Từ khóa


Tài liệu tham khảo

Shilov, 2003, Russ. Chem. Bull., 52, 2555, 10.1023/B:RUCB.0000019873.81002.60

Ertl, 2008, Angew. Chem., Int. Ed., 47, 3524, 10.1002/anie.200800480

Schrauzer, 1977, J. Am. Chem. Soc., 99, 7189, 10.1021/ja00464a015

Ranjit, 1996, J. Photochem. Photobiol., A, 96, 181, 10.1016/1010-6030(95)04290-3

Rusina, 2003, Chem.–Eur. J., 9, 561, 10.1002/chem.200390059

Hoshino, 2001, Chem.–Eur. J., 7, 2727, 10.1002/1521-3765(20010702)7:13<2727::AID-CHEM2727>3.0.CO;2-4

Hoshino, 2000, Angew. Chem., Int. Ed., 39, 2509, 10.1002/1521-3773(20000717)39:14<2509::AID-ANIE2509>3.0.CO;2-I

Zhao, 2014, Appl. Catal., B, 144, 468, 10.1016/j.apcatb.2013.07.047

Kitano, 2012, Nat. Chem., 4, 934, 10.1038/nchem.1476

Banerjee, 2015, J. Am. Chem. Soc., 137, 2030, 10.1021/ja512491v

Zhu, 2013, Nat. Mater., 12, 836, 10.1038/nmat3696

Yandulov, 2003, Science, 301, 76, 10.1126/science.1085326

Li, 2015, J. Am. Chem. Soc., 137, 6393, 10.1021/jacs.5b03105

Hu, 2013, Angew. Chem., Int. Ed., 52, 5636, 10.1002/anie.201301709

Zhang, 2013, Small, 9, 996, 10.1002/smll.201202156

Li, 2011, J. Am. Chem. Soc., 133, 10878, 10.1021/ja2025454

Lu, 2014, Phys. Chem. Chem. Phys., 16, 21280, 10.1039/C4CP02846E

Qiao, 2016, Mater. Lett., 169, 241, 10.1016/j.matlet.2016.01.093

Balayeva, 2016, Mater. Res. Bull., 75, 155, 10.1016/j.materresbull.2015.11.037

Hong, 2013, J. Mater. Chem. A, 1, 11754, 10.1039/c3ta12332d

Yang, 2015, Appl. Catal., B, 170–171, 225, 10.1016/j.apcatb.2015.01.046

Oregan, 1991, Nature, 353, 737, 10.1038/353737a0

Ding, 2015, Appl. Surf. Sci., 357, 1606, 10.1016/j.apsusc.2015.10.030

Chen, 2004, Chem. Lett., 33, 1294, 10.1246/cl.2004.1294

Nakajima, 2005, Chem. Phys. Lett., 409, 81, 10.1016/j.cplett.2005.04.093

Shi, 2007, J. Phys. Chem. C, 111, 693, 10.1021/jp065744z