Nanostructured Oxide Catalysts for Oxidative Activation of Alkanes

Topics in Catalysis - Tập 52 - Trang 962-969 - 2009
V. Cortés Corberán1
1Institute of Catalysis and Petroleumchemistry, CSIC, Madrid, Spain

Tóm tắt

The valorization of light alkanes via catalytic oxidative dehydrogenation (ODH) and selective oxidation is, with a few exemptions, still not solved. Oxide catalysts play a foremost role in these reactions. The control of the nanostructure brings new ways to tune their catalytic properties, but to date this has been little explored for alkane activation. This paper offers an overview of the applications of nanostructured oxide catalysts to oxidative activation of alkanes. Relevant examples of their unusual performance, the improvement of activity and selectivity attained by these oxides, and the new features brought by ordered mesoporous oxides, are discussed. Application of nanotechnology to oxides brings both new challenges and opportunities for catalytic applications. To make the most of it, a broad multidisciplinary approach, and bridging the lack of communication among the various research areas (electronics, materials, catalysis) involved, are needed.

Tài liệu tham khảo

Boulding KE (1966) In: Jarrett H (ed) Environmental quality in a growing economy. John Hopkins, Baltimore Cavani F, Trifirò F (1995) Catal Today 24:307 Cavani F, Trifirò F (1992) Appl Catal 88:115 Mamedov EA, Cortés Corberán V (1995) Appl Catal 127:1 Haruta M, Kobayashi T, Sano H, Yamada N (1987) Chem Lett 2:405 Hayashi T, Tanaka K, Haruta M (1998) J Catal 178:566 Boccuzzi F, Chiorino A, Manzoli M, Lu P, Akita T, Ichikawa S, Haruta M (2001) J Catal 202:256 Lee YNg, El-Fadli Z, Sapiña F, Martínez-Tamayo E, Cortés Corberán V (1999) Catal Today 52:45 Lee YNg, Sapiña F, Martínez E, Folgado JV, Cortés Corberán V (1997) Stud Surf Sci Catal 110:747 Nakamura T, Misono M, Uchijima T, Yoneda Y (1980) Nippon Kagaku Kaishi 679 Arai H, Yamada T, Eguchi K, Seiyama T (1986) Appl Catal 26:265 Madeira LM, Portela MF, Mazzocchia C (2004) Catal Rev 46:53 Valenzuela RX, Bueno Sobrino G, Vie Giner D, Martínez E, Sapiña F, Cortés Corberán V (2001) Book of extended abstracts. In: IV world congress on catalytic oxidation, vol II, Berlin-Postdam, p 213 Vie D, Martínez E, Sapiña F, Folgado JV, Beltrán A, Valenzuela RX, Cortés Corberán V (2004) Chem Mater 16:1697 He Y, Wu Y, Chen T, Weng WZ, Wan HL (2006) Catal Commun 7:268 Wu Y, He Y, Chen T, Weng WZ, Wan HL (2006) Appl Surf Sci 252:5220 Davies TE, García T, Solsona B, Taylor SH (2006) Chem Commun 3417 Cortés Corberán V (2005) Catal Today 99:33 Valenzuela RX, Bueno G, Cortés Corberán V, Xu Y, Chen C (2000) Catal Today 61:43 Valenzuela RX, Bueno G, Solbes A, Sapiña F, Martínez E, Cortés Corberán V (2001) Top Catal 15:181 Navas J, Martínez E, Sapiña F, Cortés Corberán V (2007) Book of abstracts. 8th NGCS, Natal, Brazil, May 2007, p 163 Reddy BM, Han D-S, Jiang N, Park S-E (2008) Catal Surv Asia 12:56 Deng S, Li HQ, Zhang Y (2003) Chin J Catal 24:744 Deng S, Li HQ, Li S, Zhang Y (2007) J Mol Catal A Chem 268:169 Bi YL, Cortés Corberán V, Zhuang H, Zhen K-J (2004) Stud Surf Sci Catal 153:343 Takehira K, Ohishi Y, Shishido T, Takaki K, Zhang Q, Wang Y (2004) Stud Surf Sci Catal 153:323 Valenzuela RX, Cortés Corberán V (2000) Top Catal 11/12:153 Jia MJ, Valenzuela RX, Amorós P, Beltrán-Porter D, El-Haskouri J, Marcos MD, Cortés Corberán V (2004) Catal Today 91–92:43 Huerta LJ, Amorós P, Beltrán-Porter D, Cortés Corberán V (2006) Catal Today 117:180 Hess C, Looi MH, Hamid SBA, Schlögl R (2006) Chem Commun 451–453 Cortés Corberán V, Jia MJ, El-Haskouri J, Valenzuela RX, Beltrán-Porter D, Amorós P (2004) Catal Today 91–92:127 Li J, Armor JN (1998) J Catal 173:511 Huang MH (2001) Science 292:1897 Adachi M, Murata Y, Okada I, Yoshikawa S (2003) J Electrochem Soc 150:G488 Bae C, Yoo H, Kim S, Lee K, Kim J, Sung MM, Shin H (2008) Chem Mater 20:756 Cortes-Jácome MA, Morales M, Angeles Chavez C, Ramírez-Verduzco LF, López-Salinas E, Toledo-Antonio JA (2007) Chem Mater 19:6605