Methods for calculating of the speed of sound in layering saline binary mixtures

Pleiades Publishing Ltd - Tập 85 - Trang 1850-1854 - 2011
A. R. Zinatulina1, N. K. Tkachev1
1Institute of High Temperature Electrochemistry, Russian Academy of Sciences, Ural Branch, Yekaterinburg, Russia

Tóm tắt

We develop a method for calculating the speed of sound and the compressibility of layered saline melts based on two approximations of the statistical theory of many-sorted ion systems, predicting the existence of an immiscibility cupola. Good agreement is observed between the kind of temperature dependency of the speed of sound in the monophase and diphase areas and experimental data both in a modified Debye-Hückel theory and in a mean spherical approximation. Improvement in the quantitative predictions for the mean spherical approximation with specific permittivity estimated on the basis of experimental data on the refractive index is established.

Tài liệu tham khảo

A. D. Bergman, E. L. Kazachenko, and S. I. Berezina, Zh. Neorg. Khim. 9, 1214 (1964). M. L. Sholokhovich, D. S. Lesnykh, G. A. Bukhalova, and A. D. Bergman, Dokl. Akad. Nauk SSSR 103, 261 (1955). C. Margheritis, G. Flor, and C. Sinistri, Z. Naturforsch., A: Phys. Sci. 28, 1329 (1973). N. K. Tkachev, I. V. Rukavishnikova, V. N. Lokket, and V. P. Stepanov, Elektrokhimiya 43, 1004 (2007) [Russ. J. Electrochem. 43, 955 (2007)]. V. N. Lockett, I. V. Rukavishnikova, V. P. Stepanov, and N. K. Tkachev, Phys. Chem. Chem. Phys., No. 12, 1139 (2010). V. P. Stepanov and V. I. Minchenko, Zh. Fiz. Khim. 83, 147 (2009) [Russ. J. Phys. Chem. A 83, 129 (2009)]. N. K. Tkachev, Dokl. Akad. Nauk 362, 75 (1998) [Dokl. Chem. 362, 164 (1998)]. A. R. Zinatulina and N. K. Tkachev, Rasplavy, No. 2, 68 (2010). G. A. Mansoori, N. F. Carnahan, K. E. Starling, and T. W. Leland, J. Chem. Phys. 54, 1523 (1971). P. Debye, Selected Works (Nauka, Leningrad, 1987), p. 559 [in Russian]. L. Blum, Mol. Phys. 30, 1529 (1975). L. Blum, J. Phys. Chem. 81, 1311 (1977). L. D. Landau and E. M. Lifshitz, Course of Theoretical Physics, Vol. 6: Fluid Mechanics (Nauka, Moscow, 1986; Pergamon, New York, 1987). L. D. Landau and E. M. Lifshitz, Course of Theoretical Physics, Vol. 5: Statistical Physics (Nauka, Moscow, 1995; Pergamon, Oxford, 1980). M. P. Tosi and F. G. Fumi, J. Phys. Chem. Solids 25, 45 (1964). P.-G. de Gennes, Scaling Concepts in Polymer Physics (Cornell Univ., Ithaca, London, 1979; Mir, Moscow, 1982). V. A. Kochedykov and V. A. Khokhlov, Rasplavy, No. 6, 22 (2000).