Infrared study of goethites of varying crystallinity and particle size: I. Interpretation of OH and lattice vibration frequencies

Clay Minerals - Tập 21 Số 2 - Trang 191-200 - 1986
Philippe Cambier1
1INRA, Versailles, France

Tóm tắt

Abstract

A detailed study of the IR spectrum of goethite is given with the aim of relating variations to crystalline order and particle size. The OH stretching vibrations are split into two active components at high frequency, plus two inactive ones at low frequency. Two different bending modes exist from site group splitting. Their active modes from factor group splitting are at lower frequencies than the uncoupled ones. The lattice bands at 630 and 400 cm−1 correspond to Fe-O or Fe-OH stretching, approximately parallel to a and c, and thus respectively sensitive and not sensitive to the particle shape, as long as it remains elongated along c.

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Tài liệu tham khảo

10.1346/CCMN.1981.0290202

10.1180/mono-4

10.1103/PhysRevB.14.1715

10.1016/0022-2860(82)85065-5

10.1016/0584-8539(73)80115-1

10.1088/0022-3719/13/8/022

10.1180/claymin.1981.016.4.06

10.1346/CCMN.1985.0330501

10.1346/CCMN.1979.0270507

10.1180/claymin.1970.008.3.02

10.1002/zaac.19633260111

Kolesova, 1962, IR absorption spectroscopy of αAlOOH, γAlOOH and GaOOH, Zhurnal struktumoi Khimii, 3, 680

Cabannes-Ott, 1957, Sur la structure de quelques hydroxydes naturels: diaspore, manganite, goethite, lépidocrocite, C.R. Acad. Sci., Paris, 244, 2491

10.1088/0022-3719/1/1/321

10.1180/claymin.1986.021.2.09

Isetti, 1969, Studio sul pleocroismo infrarosso del diasporo, Periodico Mineral. Roma, 38, 31

10.1180/claymin.1977.012.02.07

10.1088/0034-4885/33/1/304

10.2320/jinstmet1952.33.12_1371

10.1180/claymin.1984.019.4.02

Schwarzmann, 1969, Die Wasserstoffbrückenbindung in Hydroxiden mit Diasporstruktur, Z. Naturforschg., 24, 8, 10.1515/znb-1969-0105