Hydrothermal Synthesis of MoS2/rGO Heterostructures for Photocatalytic Degradation of Rhodamine B under Visible Light

Journal of Nanomaterials - Tập 2021 - Trang 1-11 - 2021
Thi Thuy Trang Phan1, Thi Thanh Huong Nguyen1, Ha Tran Huu2, Thanh Tam Truong1, Le Tuan Nguyen1, Van Thang Nguyen2,1, Vy Anh Tran3,4, Thi Lan Huong Nguyen1, Hồng Liên Nguyễn5, Vien Vo2,1
1Faculty of Natural Sciences, Quy Nhon University, Quy Nhon 55000, Vietnam
2Applied Research Institute for Science and Technology, Quy Nhon University, Quy Nhon 55000, Vietnam
3Faculty of Environmental and Chemical Engineering, Duy Tan University, Da Nang 50000, Vietnam
4Institute of Research and Development, Duy Tan University, Da Nang 50000, Vietnam
5School of Chemical Engineering, Hanoi University of Science and Technology, Hanoi 100000, Vietnam

Tóm tắt

MoS2/rGO composites were synthesized by hydrothermal method from the precursors of MoS2 and reduced graphene oxide (rGO) prepared in the former steps. The influence of the synthesis conditions including hydrothermal temperature and mass ratio of MoS2 to rGO on the structure, morphology, and optical absorption capacity of the MoS2/rGO composites was systematically investigated using physicochemical characterizations. The photocatalytic performance of as-prepared samples was investigated on the degradation of Rhodamine B under visible light, in which, the composites obtained at hydrothermal temperature of 180°C and MoS2/rGO mass ratio of 4/1 exhibited the highest photodegradation efficiency of approx. 80% after 4 hours of reaction. This enhancement in photocatalytic behaviour of composites could be assigned to the positive effect of rGO in life time expansion of photoinduced electrons—holes.

Từ khóa


Tài liệu tham khảo

10.1016/j.jcat.2019.01.023

10.1016/j.jwpe.2019.101035

10.1016/j.mseb.2020.114678

10.1016/j.ceramint.2018.12.198

10.1016/j.watres.2010.02.039

R. Ameta, 2013, Photocatalytic Degradation of Organic Pollutants: A Review, Materials Science Forum, 247

10.1016/j.jclepro.2021.126122

10.1016/j.jphotochem.2018.09.049

10.1016/j.jpowsour.2020.229081

10.1016/j.cej.2017.09.153

10.1016/0021-9517(86)90083-7

10.1016/j.jphotochem.2013.04.015

10.1002/slct.202004337

10.1016/j.apcatb.2020.119785

10.1016/j.cej.2020.126498

10.1016/j.apsusc.2020.148159

10.1039/C6RA10923C

10.1021/jp3093786

10.1016/j.ijhydene.2014.10.129

10.1126/science.1156965

S. P. Lonkar, 2014, Applications of graphene in catalysis, Journal of Thermodynamics & Catalysis, 5, article 100132

10.1016/j.carbon.2011.11.010

10.1039/C6RA01591C

10.1155/2020/6285484

10.1007/s13391-019-00175-2

10.1016/j.jallcom.2019.02.246

10.1186/s11671-017-2248-9

10.1039/C6RA02610A

C. Koventhan, 2020, Efficient hydrothermal synthesis of flake-like molybdenum disulfide for selective electrochemical detection of metol in water real samples, International Journal of Electrochemical Science, 15, 7390, 10.20964/2020.08.43

10.1063/1.4961883

10.1166/jnn.2017.13845

10.1016/j.rinp.2019.102458

10.1016/j.scib.2017.05.025

F. A. Aisien, 2013, Photocatalytic decolourisation of industrial wastewater from a soft drink company, Journal of Engineering and Applied Science, 9, 11

10.1186/s11671-019-2916-z

10.1016/j.snb.2017.05.060

10.1016/j.jpowsour.2016.01.081

10.1016/j.electacta.2014.11.034

10.1039/C6RA15944C