Fluoride removal on Fe–Al-impregnated granular ceramic adsorbent from aqueous solution

Springer Science and Business Media LLC - Tập 16 - Trang 609-617 - 2013
Nan Chen1,2, Chuanping Feng1,2, Miao Li3
1Key Laboratory of Groundwater Cycle and Environment Evolution, Ministry of Education, China University of Geosciences (Beijing), Beijing, China
2School of Water Resources and Environment, China University of Geosciences (Beijing), Beijing, China
3School of Environment, Tsinghua University, Beijing, China

Tóm tắt

A novel Fe–Al-impregnated granular ceramic adsorbent has been developed for fluoride removal from aqueous solution. Batch experiments were performed to investigate the effect of contact time, initial pH, adsorbent dose, and the presence of competing anions on the adsorption of fluoride. More than 96 % removal of fluoride was achieved within 48 h from 10 mg/L initial fluoride solution at neutral pH. The adsorption process was well explained with pseudo-second-order and pore diffusion models. The maximum adsorption capacity of adsorbent for fluoride removal was 3.56 mg/g according to the Langmuir isotherm model. The optimum fluoride removal efficiency was observed between pH ranged of 4.0–9.0. The fluoride removal efficiency was significantly decreased in the presence of carbonate and phosphate anions. Results from this study demonstrated potential utility of Fe–Al-impregnated granular ceramic adsorbent that could be developed into a viable method for fluoride removal from aqueous solution.

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