Effects of temperature on factors relevant to laser operation near 1.6 µm wavelength in resonantly (in-band) pumped CaF2:Er and SrF2:Er crystals: a comparative study

Applied Physics B - Tập 129 - Trang 1-10 - 2023
R. Lisiecki1, B. Macalik1, J. Komar1, R. Kowalski1, A. Strzep1,2, Zhen Zhang2, Zhonghan Zhang2, Yunfei Wang2, Liangbi Su2, W. Ryba-Romanowski1
1Institute of Low Temperature and Structure Research, Polish Academy of Sciences, Wroclaw, Poland
2Key Laboratory of Transparent and Opto-functional Inorganic Materials, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai, China

Tóm tắt

Single crystals of CaF2 and SrF2 containing Er3+ ions with concentrations between 0.01 and 0.6 at% respectively, were grown using the temperature gradient technique (TGT). Absorption spectra related to the 4I15/2 → 4I13/2 transition of Er3+ ions were measured at 5 K to investigate the properties of the crystal field splitting of the 4I13/2 multiplet, and at several temperatures in the region 80 K – 300 K to determine the effect of temperature on the spectral bands. The 4I13/2 → 4I15/2 luminescence spectra were recorded within the same temperature range as for absorption measurement. The analysis of absorption and luminescence spectra provides an in-depth knowledge on the effect of temperature on the factors that govern the efficiency of resonant optical pumping near 1.6 µm and the resulting lasing ability of Er3+ ions imbedded in CaF2 and SrF2 hosts.

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