Black phosphorus nanosheets-based effective electrochemical sensor for uric acid detection

Carbon Letters - Tập 33 - Trang 2161-2169 - 2023
Hao Wang1, Haitao Wang1, Jingjing Yang1, Pramitha Yuniar Diah Maulida2, Jing Zou1, Arramel2, Can Wu3,4, Jizhou Jiang1
1School of Chemistry and Environmental Engineering, School of Materials Science and Engineering, School of Environmental Ecology and Biological Engineering, Key Laboratory of Green Chemical Engineering Process of Ministry of Education, Engineering Research Center of Phosphorus Resources Development and Utilization of Ministry of Education, Novel Catalytic Materials of Hubei Engineering Research Center, Wuhan Institute of Technology, Wuhan, China
2Nano Center Indonesia, Jalan Raya PUSPIPTEK, South Tangerang, Indonesia
3Hubei Jiangxia Laboratory, Wuhan, China
4College of Health Science and Engineering, Hubei University, Wuhan, China

Tóm tắt

Black phosphorus (BP) is incorporated in the electrochemical detection of uric acid (UA) to form few layers of BP nanosheets (BPNS)-modified glassy carbon electrodes (BPNS/GCE), investigated by means of ultrasound-assisted liquid-phase exfoliation. We find a significant increase in the peak current magnitude and positive potential shift in the electrochemical response of BPNS/GCE, which may be attributed to the larger specific surface area and good charge transfer ability of BPNS. Further, the electrochemical response of BPNS/GCE is evaluated under different conditions to achieve the optimal conditions. UA detection using differential pulse voltammetry (DPV) shows linear response within the range of 1–1000 μM with a detection limit of 0.33 μM. This work reveals new applications of BP nanomaterials in the electrochemical sensing, thereby promoting further advancement in terms of practical applications of two-dimensional nanomaterials.

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