Air Electrodes for Flexible and Rechargeable Zn−Air Batteries

SMALL STRUCTURES - Tập 3 Số 1 - 2022
Xiao Xia Wang1,2, Xiaoxuan Yang3, Hui Liu4, Tao Han5, Junhua Hu5, Hongbo Li6, Gang Wu3
1Department of Chemical and Biological Engineering University at Buffalo The State University of New York Buffalo NY 14260 USA
2Department of Chemical and Biological Engineering University at Buffalo The State University of New York Buffalo NY 14260 USA; School of Mechanical and Power Engineering East China University of Science and Technology Shanghai 200237 China
3Department of Chemical and Biological Engineering University at Buffalo The State University of New York Buffalo NY 14260 USA
4Shanghai Power and Energy Storage Battery System Engineering Tech. Co. Ltd. Shanghai 200241 China
5School of Mechanical and Power Engineering, East China University of Science and Technology, Shanghai, 200237, China
6School of Materials Science and Engineering, East China University of Science and Technology, Shanghai, 200237, China

Tóm tắt

Rechargeable Zn−air batteries (ZABs) have attracted increasing attention as one of the most promising future energy power sources due to their relatively high specific energy density, environmental friendliness, safety, and low cost. In particular, flexible ZABs are desirable for portable and wearable electronic devices, in which the cathode can utilize air directly from the atmosphere with significantly enhanced energy density. Therefore, the air electrode consisting of oxygen electrocatalysts is the most critical component in flexible ZABs, significantly governing the overall battery performance and cost. This review highlights recent achievements in designing efficient oxygen electrocatalysts and air electrodes for rechargeable and flexible ZABs. First, the most significant innovations of recent battery configurations to improve flexibility and battery performance are introduced. Then, oxygen electrocatalysts developed for fabricating high‐performance air cathodes in flexible ZABs in terms of catalyst properties, unique nanostructures, and morphologies are emphasized. Furthermore, effective architectures of air electrodes are discussed to highlight structural stability and charge/mass transports for improving battery performance. Finally, a perspective for designing durable and high‐power air electrodes for flexible ZABs is provided, aiming to summarize current challenges and possible solutions to commercialize the exciting battery technology eventually.

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