Adsorption of Ammonium by Graphene Oxide-Based Composites Prepared by UV Irradiation and Using as Slow-Release Fertilizer

Journal of Polymers and the Environment - Tập 26 - Trang 4311-4320 - 2018
Chengyi Wu1,2, Xu Zhang1, Cong Li1, Chao Cheng1, Yin Zheng1
1Department of Chemistry and Environmental Engineering, Hubei University for Nationalities, Enshi, China
2Key Laboratory of Biologic Resources Protection and Utilization of Hubei Province, Enshi, China

Tóm tắt

A novel sodium alginate-grafted poly(acrylic acid)/graphene oxide (NaAlg-g-PAA/GO) composite hydrogel was prepared via ultraviolet irradiation, and characterized by infrared spectroscopy spectrometer. X-ray diffraction, X-ray photoelectron spectroscopy and scanning electron microscopy. It was employed to adsorb NH4+ from aqueous solution and used as slow-release nitrogen fertilizers (SNFs). Result indicated that the adsorption process for NH4+ reached equilibrium within 50 min, with the adsorption capacity of 6.6 mmol g−1 even if 30 wt% GO was incorporated. The results of adsorption kinetic and isotherm were well described by the pseudo-second-order and Freundlich model. The thermodynamics analysis showed the adsorption process was spontaneous. The study indicated excellent water-holding ratio of soil with 2 wt% SNFs was 81.2%, and nitrogen release was up to 55.1% within 40 days in soil. Overall, NaAlg-g-PAA/GO could be considered as an efficient adsorbent for the recovery of nitrogen with the agronomic reuse as a fertilizer.

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