The obstruction factor γ in gas chromatography

Springer Science and Business Media LLC - Tập 14 - Trang 576-578 - 1981
P. Thumneum1, S. Hawkes1
1Department of Chemistry, Oregon State University,Corvallis,USA.

Tóm tắt

The relationship between the obstructive factor γ and velocity was restudied. The dependence of the obstructive factor on velocity was verified. The effects of diffusion coefficient and particle-to-column diameter ratio on the obstructive factor-velocity relationship were investigated. The results are consistent with Hawkes' hypothesis that values of γ at low velocities are averages over tightly packed and loosely packed domains while at high velocities they are weighted in favour of the loosely packed domains where there is more flow.

Tài liệu tham khảo

S. J. Hawkes, Anal. Chem.44, 1296 (1972). W. Bowers andS. J. Hawkes, J. Chromatogr.134, 166–169 (1977). J. H. Knox andL. McLaren, Anal. Chem.36, 1477 (1964). F. J. Yang, S. J. Hawkes, F. T. Lindstrom, J. Am. Chem. Soc.98, 5101 (1976). E. R. Bennett andW. E. Bolch, Anal. Chem.43, 55 (1971). M. A. D. Fluendy andD. S. Horne, Separ. Sci.3, 203 (1968). D. D. Chilcote andC. D. Scott J. Chromatogr.87, 315 (1973). M. R. Edwards andJ. F. Richardson, Chem. Eng. Sci.23, 109 (1968). S. J. Hawkes andS. P. Steed, J. Chromatogr. Sci.8, 256 (1970). L. Schanel andP. Schneider, Chem Eng. J.2, 274 (1971). G. H. Neale andW. K. Nader, J. Ameri. Int. Chem Eng.19, 112 (1973). T. R. Marrero andE. A. Mason, J. Phys. Chem. Ref. Data, 1, 3 (1972). J. C. Sternberg andR. E. Poulson, Anal. Chem.36, 58 (1964). J. C. Giddings, Dynamics of Chromatography, Part I Principles and Theory, Marcel Dekker, Inc. New York, p. 247 (1965).