Experimental and theoretical studies (DFT) on technetium extraction as HTcO4 using dicyclohexano-18-crown-6 in a blend of isodecyl alcohol and n-dodecane from acidic medium

Progress in Nuclear Energy - Tập 160 - Trang 104684 - 2023
Pasupati Nath Khan1,2, Prithwish Sinharoy1, A. Bhattacharyya2,3
1Nuclear Recycle Group, Bhabha Atomic Research Centre, Mumbai, 400085, India
2Homi Bhabha National Institute, Anushaktinagar, Mumbai 400094, India
3Radio Chemistry Division, Bhabha Atomic Research Centre, Mumbai 400085, India

Tài liệu tham khảo

Ali, 2011, Selective extraction of perrehnate anion in nitric acid solution using 2,2′-(methylimino)bis(N, N′-diethylacetamide) as an extractant, Prog. Nucl. Energy, 53, 1005, 10.1016/j.pnucene.2011.05.011 Ali, 2012, Selective extraction of perrhenate anion in nitric acid solution using 2,2 ’-(imino)bis(N, N’-dioctylacetamide) as an extractant, Sep. Purif. Technol., 92, 77, 10.1016/j.seppur.2012.03.021 Becke, 1988, Density-functional exchange-energy approximation with correct asymptotic behavior, Phys. Rev. A, 38, 3098, 10.1103/PhysRevA.38.3098 Becke, 1992, Density‐functional thermo chemistry. III. The role of exact exchange-only gradient correction, J. Chem. Phys., 96, 2155, 10.1063/1.462066 Bonnesen, 1996 Denniss, 1996, Reprocessing irradiated fuel Dileep, 2008, Distribution of technetium in PUREX process streams, Desalination, 232, 157, 10.1016/j.desal.2007.11.053 El Kalai, 2019, New organic extractant based on pyridazinone scaffold compounds: liquid-liquid extraction study and DFT calculations, J. Mol. Struct., 1191, 24, 10.1016/j.molstruc.2019.04.033 Favre-Réguillon, 2019, Insights in uranium extraction from spent nuclear fuels using dicyclohexano-18-crown-6 – fate of rhenium as technetium homolog, Sep. Purif. Technol., 209, 338, 10.1016/j.seppur.2018.07.034 George, 2022, A review of technetium and zirconium extraction into tributyl phosphate in the PUREX process, Hydrometallurgy, 211, 10.1016/j.hydromet.2022.105892 Ihsanullah, 1993, Losses of technetium during various steps in the development of a procedure for environmental samples, J. Radioanal. Nucl. Chem., 176, 303, 10.1007/BF02163495 Jalhoom, 1986, Extraction of technetium by crown ethers and cryptands, J. Radioanal. Nucl. Chem., 104, 131, 10.1007/BF02163256 Kim, 2018, Volatile species of technetium and rhenium during waste vitrification, J. Non-Cryst. Solids, 481, 41, 10.1016/j.jnoncrysol.2017.10.013 Kumar, 2012, Separation of strontium from the raffinate solution of TEHDGA-actinide partitioning process: batch extraction and process development, Sep. Purif. Technol., 98, 118, 10.1016/j.seppur.2012.07.007 Lee, 1988, Development of the Colle-Salvetti correlation-energy formula into a functional of the electron density, Phys. Rev. B: Condens. Matter Mater. Phys., 37, 785, 10.1103/PhysRevB.37.785 Leonard, 1999, Developing and testing an alkaline-side solvent extraction process for technetium separation from tank waste, Separ. Sci. Technol., 34, 1043, 10.1080/01496399908951080 Manohar, 2007, Process Development for Bulk Separation of trivalent actinides and lanthanides from radioactive high-level liquid waste, Nucl. Sci. Eng., 156, 96, 10.13182/NSE07-A2688 Melent’ev, 2011, Effect of some reducing and complexing agents on the extraction behavior of technetium in the TBP-HNO3 system, Radiochemistry, 53, 256, 10.1134/S1066362211030052 Minh, 1988, Extraction of technetium from ascorbic acid medium with crown ethers, J. Radioanal. Nucl. Chem., 128, 417, 10.1007/BF02205197 Perdew, 1986, Density-functional approximation for the correlation energy of the inhomogeneous electron gas, Phys. Rev. B, 33, 8822, 10.1103/PhysRevB.33.8822 Popova, 2003, Technetium behaviour during reprocessing of spent nuclear fuel and in environmental objects, Russ. Chem. Rev., 72, 101, 10.1070/RC2003v072n02ABEH000785 Pruett, 1981, The solvent extraction of heptavalent technetium by tributyl phosphate, Separ. Sci. Technol., 16, 1157, 10.1080/01496398108057605 Raj, 2006, Radioactive waste management practices in India, Nucl. Eng. Des., 236, 914, 10.1016/j.nucengdes.2005.09.036 Ramanujam, 2001, 7918 Saeki, 2012, Structural study on 2,2 ’-(Methylimino)bis(N, NDioctylacetamide) complex with Re(VII)O4− and Tc(VII)O4− by 1H NMR, EXAFS, and IR spectroscopy, Inorg. Chem., 51, 5814, 10.1021/ic3003405 Sasaki, 2007, Highly selective extraction of TcO4−, ReO4−, and MoO42− by the new ligand, 2,2′-(methylimino)bis(N, N-dioctylacetamide) (MIDOA), Chem. Lett., 36, 1394, 10.1246/cl.2007.1394 Sasaki, 2009, 2,2’-(Methylimino)bis(N, ndioctylacetamide) (MIDOA), A new tridentate extractant for technetium(VII), rhenium(VII), palladium(II), and plutonium(IV), solvent extr, Ion Exch, 27, 378, 10.1080/07366290902821248 Sasaki, 2011, Technetium(VII) and rhenium (VII) extraction by a new diamide reagent, 2,2’-(imino)bis(N,N-dialkylacetamide) (IDAA), solvent extr, Res. Dev. J., 18, 69 Sasaki, 2013, Extraction behavior of metal ions by TODGA, DOODA, MIDOA, and NTAamide extractants from HNO3 to n-dodecane, solvent extr, Ion Exch, 31, 401, 10.1080/07366299.2013.800431 Sasaki, 2014, Complexing agents for oxonium anions of Mo and Re and their masking effects on extraction using N-donor extractants, Chem. Lett., 43, 1538, 10.1246/cl.140502 Sasaki, 2015, Studies on the extraction of soft acid metal species using MIDOA and analogous compounds, Solvent Extr. Res. Dev., Jpn., 22, 37, 10.15261/serdj.22.37 Sasaki, 2016, Masking effects for Mo, Re, Pd and Ru by S and N-donor reagents through MIDOA and ntaamide extraction, Solvent Extr. Res. Dev., Jpn., 23, 161, 10.15261/serdj.23.161 Schäfer, 1994, Fully optimized contracted Gaussian basis sets of triple zeta valence quality for atoms Li to Kr, J. Chem. Phys., 100, 5829, 10.1063/1.467146 Schulz, 1990 Sekine, 1993, Application of laser induced photoacoustic spectroscopy to the determination of99Tc, J. Nucl. Sci. Technol., 30, 1131, 10.1080/18811248.1993.9734598 Sharma, 2014, Process development for separation of cesium from acidic nuclear waste solution using 1,3-dioctyloxycalix[4]arene-crown-6+isodecyl alcohol/n-dodecane solvent, Sep. Purif. Technol., 135, 176, 10.1016/j.seppur.2014.08.016 Sharma, 2018, Process for separation of technetium from alkaline low level waste using di-tert-butyldibenzo-18-crown-6 + isodecyl alcohol/n-dodecane solvent, Sep. Purif. Technol., 207, 416, 10.1016/j.seppur.2018.04.058 Shimojo, 2020, Solvent extraction of technetium(VII) and rhenium(VII) using a hexaoctylnitrilotriacetamide extractant, Anal. Sci., 36, 1435, 10.2116/analsci.20C014 Shu, 2022, Synthesis of new carbazole derivative extractants and study on extraction of perrhenate/pertechnetate, Polyhedron, 214, 10.1016/j.poly.2021.115641 Sigala, 2015, Determination of hydrogen bond structure in water versus aprotic environments to test the relationship between length and stability, J. Am. Chem. Soc., 137, 5730, 10.1021/ja512980h Sonar, 2012, Analysis of 99Tc in the radioactive liquid waste after extraction into suitable solvent, J. Radioanal. Nucl. Chem., 294, 185, 10.1007/s10967-011-1583-z Szalewicz, 2003, 505 Takeuchi, 1993, Solvent extraction of Tc(VII) and Re(VII) from nitric acid Solution with the mixture of CMPO and TBP, Radiochim. Acta, 63, 97, 10.1524/ract.1993.63.special-issue.97 Takeuchi, 1995, Reaction stoichiometry for coextraction of technetium (VII) with uranium(VI) by CMPO, J. Radioanal. Nucl. Chem., 191, 189, 10.1007/BF02035997 Thevenet, 2018, Syntheses and evaluation of new hydrophilic azacryptands used as masking agents of technetium in solvent extraction processes, Dalton Trans., 50, 1620, 10.1039/D0DT04210B Thevenet, 2020, Perrhenate and pertechnetate complexation by an azacryptand in nitric acid medium, Dalton Trans., 49, 1446, 10.1039/C9DT04314D Tian, 2005, Extraction of actinide(III, IV, V, VI) ions and TcO4 − by N, N, N′, N′-Tetraisobutyl-3-Oxa-Glutaramide, solvent extr, Ion Exch, 23, 631, 10.1081/SEI-200068518 Wang, 2020, Efficient separation of perrhenate as analogue to pertechnetate in nitric acid solution with a DOTA-tetraamide ligand: solvent extraction, complexation and structure study, J. Mol. Struct., 1216, 10.1016/j.molstruc.2020.128330 Wang, 2021, A H-bonding and electrostatic interaction combined strategy for TcO4− separation by a nitrotriacetate-derived amine-amide extractant, Inorg. Chem., 60, 10899, 10.1021/acs.inorgchem.1c00111 Weigend, 2005, Balanced basis sets of split valence, triple zeta valence and quadruple zeta valence quality for H to Rn: design and assessment of accuracy, Phys. Chem. Chem. Phys., 7, 3297, 10.1039/b508541a Wilmarth, 2011, Review: waste pretreatment technologies for remediation of legacy defense nuclear wastes, Solvent Extr. Ion Exch., 29, 1, 10.1080/07366299.2011.539134