4-dimethylaminopyridine-catalyzed cascade reaction for efficient synthesis of naphthofurans

Chemical Research in Chinese Universities - Tập 32 - Trang 62-67 - 2016
Chenli Fan1,2, Xinwei He2, Kaisheng Liao2, Cui’e Wang2, Yongjia Shang2
1Department of Material Engineering, Wuhu Institute of Technology, Wuhu, P. R. China
2Key Laboratory of Functional Molecular Solids, Ministry of Education, Anhui Key Laboratory of Molecule-based Materials, College of Chemistry and Materials Science, Anhui Normal University, Wuhu, P. R. China

Tóm tắt

A convenient and efficient method was developed for the synthesis of naphtho[2,1-b]furans via 4-dimethylaminopyridine(DMAP)-catalyzed cascade reaction of 2-hydroxy-1-naphthaldehydes and α-halogenated ketones in moderate to good yields in the presence of Na2CO3 at 80 ºC for 6 h. The mechanism for this process was briefly discussed with a tentative catalytic cycle proposed. Moreover, this method features organocatalysts and high step-economy, which make it practical and attractive.

Tài liệu tham khảo

Srivastava V., Negi A. S., Kumar J. K., Faridi U., Sisodia B. S., Darokar M. P., Luqman S., Khanuja S. P. S., Bioorg. Med. Chem. Lett., 2006, 16(4), 911 Rao V. K., Shelke G. M., Tiwari R., Parang K., Kumar A., Org. Lett., 2013, 15(9), 2190 Le Guével R., Oger F., Lecorgne A., Dudasova Z., Chevance S., Bondon A., Barath P., Simonneaux G., Salbert G., Bioorg. Med. Chem., 2009, 17(19), 7021 Gan C. S., Nan D. D., Qiao J. P., Wang C. W., Zhou J. N., J. Nucl. Med., 2012, 53(Sup.1), 1620 Zeni G., Larock R. C., Chem. Rev., 2006, 106(11), 4644 Patil N. T., Yamamoto Y., Chem. Rev., 2008, 108(8), 3395 Butin A. V., Melchin V. V., Abaev V. T., Bender W., Pilipenko A. S., Krapivin G. D., Tetrahedron, 2006, 62(34), 8045 Park K. K., Jeong J., Tetrahedron, 2005, 61(3), 545 Guo X., Yu R., Li H., Li Z., J. Am. Chem. Soc., 2009, 131(47), 17387 Lingam V. S. P. R., Dahale D. H., Mukkanti K., Gopalan B., Thomas A., Tetrahedron Lett., 2012, 53(42), 5695 Hou C. D., Xu X. L., An J. Z., Jia X. D., Wang X. C., Wang C., J. Org. Chem., 2012, 77(18), 8310 Hou C. D., An J. Z., Xu X. L., Jia X. D., Wang X. C., Kang L. S., Tetrahedron Lett., 2013, 54(9), 1145 France S., Guerin D. J., Miller S. J., Lectka T., Chem. Rev., 2003, 103(8), 2985 Tian S. K., Chen Y. G., Hang J., Tang L., McDaid P., Deng L., Acc. Chem. Res., 2004, 37(8), 621 Jin L. L., Lei Y. T., Chem. Res. Chinese Universities, 2013, 29(4), 710 Liu Z. M., Fang J., Yan C. G., Chem. Res. Chinese Universities, 2013, 29(6), 1089 Shang Y. J., Wang C. E., He X. W., Ju K., Zhang M., Yu S. Y., Wu J. P., Tetrahedron, 2010, 66(50), 9629 Wu J. P., Shang Y. J., Wang C. E., He X. W., Yan Z. L., Hu M. M., Zhou F. Y., RSC Adv., 2013, 3(14), 4643 Kar S., Lahiri S., Chem. Commun., 1995, (9), 957 Rao M. L. N., Awasthi D. K., Banerjee D., Tetrahedron Lett., 2007, 48(3), 431 Jakub S., Jan S., Heterocycl. Commun., 1999, 5(4), 349 Axelle A., Frédérique T., Gérald G., Synthesis, 1999, (7), 1241 Naskar S., Banerjee M., Hazra A., Mondal S., Maity A., Paira R., Sahu K. B., Saha P., Banerjee S., Mondal N. B., Tetrahedron Lett., 2011, 52, 1527