A novel photosensitizing decatungstate-based MOF: Synthesis and photocatalytic oxidation of cyclohexane with molecular oxygen

Inorganic Chemistry Communications - Tập 100 - Trang 125-128 - 2019
Dongying Shi1, Zheng Ming2, Qiuyu Wu1, Tianhua Lai1, Kaijun Zheng1, Cheng He2, Junwei Zhao3
1Henan Provincial Key Laboratory of Surface & Interface Science, Zhengzhou University of Light Industry, Zhengzhou 450002, PR China
2State Key Laboratory of Fine Chemicals, Dalian University of Technology, Dalian 116024, PR China
3Henan Key Laboratory of Polyoxometalate Chemistry, Henan University, Kaifeng 475004, PR China

Tài liệu tham khảo

Okada, 2014, Sunlight photocatalyzed regioselective β-alkylation and acylation of cyclopentanones, Chem. Sci., 5, 2893, 10.1039/C4SC01072H Ravelli, 2009, Photocatalysis. A multi-faceted concept for green chemistry, Chem. Soc. Rev., 38, 1999, 10.1039/b714786b Molinari, 2013, Photocatalytic properties of sodium decatungstate supported on sol–gel silica in the oxidation of glycerol, Catal. Today, 206, 46, 10.1016/j.cattod.2011.11.033 Molinari, 2010, Matrix effects on the photocatalytic oxidation of alcohols by [n-Bu4N]4W10O32 incorporated into sol–gel silica, Dalton Trans., 39, 7826, 10.1039/c003282d Molinari, 2007, Photocatalytic and catalytic activity of heterogenized W10O324− in the bromide-assisted bromination of arenes and alkenes in the presence of oxygen, J. Mol. Catal. A-Chem., 262, 156, 10.1016/j.molcata.2006.08.056 Ryu, 2011, Atom-economical synthesis of unsymmetrical ketones through photocatalyzed C–H activation of alkanes and coupling with CO and electrophilic alkenes, Angew. Chem. Int. Ed., 50, 1869, 10.1002/anie.201004854 Tanielian, 1998, Decatungstate photocatalysis, Coord. Chem. Rev., 178–180, 1165, 10.1016/S0010-8545(98)00160-X Maldotti, 2008, Selective photooxidation of diols with silica bound W10O324−, J. Catal., 253, 312, 10.1016/j.jcat.2007.11.008 Bigi, 2007, Silica-bound decatungstates as heterogeneous catalysts for H2O2 activation in selective sulfide oxidation, J. Catal., 250, 222, 10.1016/j.jcat.2007.06.019 Li, 2013, Decatungstate incorporated metal–organic framework for degradation of rhodamine-B under sunlight irradiation, Chinese J. Struct. Chem., 32, 1897 Sun, 2009, Highly stable crystalline catalysts based on a microporous metal–organic framework and polyoxometalates, J. Am. Chem. Soc., 131, 1883, 10.1021/ja807357r Chen, 2017, Dynamic spacer installation for multirole metal–organic frameworks: a new direction toward multifunctional MOFs achieving ultrahigh methane storage working capacity, J. Am. Chem. Soc., 139, 6034, 10.1021/jacs.7b01320 Liu, 2014, Applications of metal–organic frameworks in heterogeneous supramolecular catalysis, Chem. Soc. Rev., 43, 6011, 10.1039/C4CS00094C Wang, 2018, Polyoxometalate-based metal–organic frameworks with conductive polypyrrole for supercapacitors, ACS Appl. Mater. Interfaces, 10, 32265, 10.1021/acsami.8b12194 Shi, 2015, Merging of the photocatalysis and copper catalysis in metal–organic frameworks for oxidative C–C bond formation, Chem. Sci., 6, 1035, 10.1039/C4SC02362E Du, 2014, Recent advances in porous polyoxometalate-based metal–organic framework materials, Chem. Soc. Rev., 43, 4615, 10.1039/C3CS60404G Shi, 2016, A photosensitizing decatungstate-based MOF as heterogeneous photocatalyst for the selective C–H alkylation of aliphatic nitriles, Chem. Commun., 52, 4714, 10.1039/C6CC00862C Tzirakis, 2009, Decatungstate as an efficient photocatalyst in organic chemistry, Chem. Soc. Rev., 38, 2609, 10.1039/b812100c Molinari, 2000, Photocatalyzed oxidation of cyclohexene and cyclooctene with (n-Bu4N)4W10O32 and (n-Bu4N)4W10O32/FeIII[meso-tetrakis(2,6-dichlorophenyl)porphyrin] in homogeneous and heterogeneous systems, Eur. J. Inorg. Chem., 91, 10.1002/(SICI)1099-0682(200001)2000:1<91::AID-EJIC91>3.0.CO;2-J Fornal, 2007, Photocatalyzed oxidation of cyclohexane with heterogenized decatungstate, J. Photoch. Photobio. A, 188, 279, 10.1016/j.jphotochem.2006.12.023 Wu, 2015, (n-Bu4N)4W10O32-catalyzed selective oxygenation of cyclohexane by molecular oxygen under visible light irradiation, Appl. Catal, B-Environ., 164, 113 Spek, 1999 Shi, 2012, Four types of 1D or 2D organic–inorganic hybrids assembled by arsenotungstates and CuII–LnIII/IV heterometals, CrystEngComm, 14, 3108, 10.1039/c2ce06354a Zhao, 2012, Two organic–inorganic hybrid 1-D and 3-D polyoxotungstates constructed from hexa-CuII substituted sandwich-type arsenotungstate units, CrystEngComm, 14, 2797, 10.1039/c2ce06298d Zhao, 2011, Two 1-D multi-nickel substituted arsenotungstate aggregates, CrystEngComm, 13, 3462, 10.1039/c0ce00983k Shi, 2017, Semiconductive copper(I)–organic frameworks for efficient light-driven hydrogen generation without additional photosensitizers and cocatalysts, Angew. Chem. Int. Ed., 56, 14637, 10.1002/anie.201709869 Shi, 2016, A breathing MOF: direct crystallographic observation of the site-selective C(sp3)–H functionalization, RSC Adv., 6, 51936, 10.1039/C6RA07100G Ravelli, 2016, Decatungstate anion for photocatalyzed “window ledge” reactions, Acc. Chem. Res., 49, 2232, 10.1021/acs.accounts.6b00339 Laudadio, 2018, Selective C(sp3)–H aerobic oxidation enabled by decatungstate photocatalysis in flow, Angew. Chem. Int. Ed., 57, 4078, 10.1002/anie.201800818 Maldotti, 2002, Immobilization of (n-Bu4N)4W10O32 on mesoporous MCM-41 and amorphous silicas for photocatalytic oxidation of cycloalkanes with molecular oxygen, J. Catal., 209, 210, 10.1006/jcat.2002.3618