Crosslinking of diene polymers via ‘ENE’ reaction with bistriazolinediones

Polymer Bulletin - Tập 2 - Trang 513-520 - 1980
Swoyam P. Rout1, George B. Butler1
1Center for Macromolecular Science and Department of Chemistry, University of Florida, Gainesville, USA

Tóm tắt

Bistriazolinediones (BTDs) have been used to synthesize a large number of highly crosslinked polydienes by the ‘ene’ reaction. BTDs have been found to be effective crosslinking agents at room temperature. The crossliked polymers were swollen in benzene, and the crosslink density and the molecular weight between crosslinks were determined by the Flory-Rehner equation.

Tài liệu tham khảo

J. SAUER and B. SCHRODER, Angew.Chem.Intl.Edn.Eng. 4, 711 (1965) H. M. R. HOFFMANN, Angew.Chem.Intl.Edn.Eng., 4, 711 (1969) A. G. WILLIAMS and G. B. BUTLER, J.Polym.Sci. Polym.Chem.Ed., 17, 1117 (1979) B. SAVILLE, J.Chem.Soc., D, 12, 635 (1971) K. A. MATYJAZEWSKI, K. B. WAGENER and G.B. BUTLER, J.Polym.Sci.Polym.Lett.Ed., 17, 65 (1979) K. A. MATYJAZEWSKI, K. B. WAGENER and G. B. BUTLER, ibid. P. J. FLORY and J. REHNER, J.Chem.Phys., 11, 521 (1943) M. RUTKOWSKA and A. KWIATKOWSKI, J.Polym.Sci. Polym.Symp., 53, 141 (1975) S. R. TURNER, Doctoral Dissertation, University of Florida, Gainesville, Florida (1971) L. E. NIELSEN, J.Macromol.Sci.Rev.Macromol.Chem., C3, 69 (1969) W. L. HERGENROTHER, J.Appl.Polym.Sci., 16, 2611 (1972) I. GANCARZ and W. KASKAWSKI, J.Polym.Sci.Polym. Chem.Ed., 17, 1523 (1979)