Preparation and properties of boron nitride/epoxy composites with high thermal conductivity and electrical insulation

Journal of Materials Science: Materials in Electronics - Tập 29 - Trang 14267-14276 - 2018
Ling Weng1,2,3, HeBing Wang1, Xiaorui Zhang1,2, Lizhu Liu1,2, Hexin Zhang4
1College of Material Science and Engineering, Harbin University of Science and Technology, Harbin, People’s Republic of China
2Key Laboratory of Engineering Dielectric and Its Application, Ministry of Education, Harbin University of Science and Technology, Harbin, People’s Republic of China
3Suzhou Jufeng Electrical Insulation System Co., Ltd, Suzhou, People’s Republic of China
4College of Material Science and Chemical Engineering, Harbin Engineering University, Harbin, People’s Republic of China

Tóm tắt

A series of boron nitride/epoxy composites with high thermal conductivity have been prepared via addition of different amounts of surface modified h-BN and c-BN powders to epoxy resin matrices. The effects of h-BN and c-BN particles on the surface morphology, thermal properties, dielectric properties and mechanical properties of these composites have been analyzed systematically. These results show that the cross-sectional morphology of these composite materials become increasingly rougher as their BN content increases. The thermal conductivity of h-BN composites were higher than that of c-BN composites, with a 253% increase in thermal conductivity observed for a 20 vol% h-BN composite, whose storage modulus was also increased. The dielectric constants of the c-BN composites were slightly higher than those of h-BN composites, but the overall increases in dielectric constant for both composites were relatively small. The resistivity of the c-BN composites was higher than the c-BN composites, with their flexural strengths decreased by varying amounts, depending on their BN loadings.

Tài liệu tham khảo

J. Hou, G. Li, N. Yang et al., J. RSC Adv. 4, 44282–44290 (2014) K.C. Yung, H. Liem, J. Appl. Polym. Sci. 106, 3587–3591 (2007) S.L. Chung, J.S. Lin, J. Mol. 21, 670 (2017) B.R. Shang, X.L. Zhao, S.R. Zheng, Z.F. Wang, S.H. Qi, J. China Plast. 30, 30–34 (2016) Y.P. Mamunya, V.V. Davydenko, P. Pissis, E.V. Lebedev, J. Eur. Polym. J. 38, 1887–1897 (2002) C. Chen, D. Hubei Province (Huazhong University of Science and Technology, Wuhan, 2016) Y. Zhang, X. Hu, J.H. Zhao, K. Sheng, W.R. Cannon, J. IEEE Trans. Compon. Packag. Technol. 32, 716–723 (2009) J. Hong, J. Lee, C. Hong, E. Sang, J. Curr. Appl. Phys. 10, 359–363 (2010) T. Zhou, X. Wang, X. Liu, D. Xiong, J. Carbon 48, 1171–1176 (2010) Y. Chen, X. Gao, J. Wang, W. He, V.V. Silberschmidt, J. Appl. Polym. Sci. (2015). https://doi.org/10.1002/app.41889 A. Rybak, K. Gaska, C. Kapusta, F. Toche, V. Salles, J. Polym. Advan. Technol. 28, 1676–1682 (2017) Y. Wu, F. Li, J.Y. Hu, X. Zhou, Y. Li, J. Appl. Polym. Sci. 19 (2015) J.P. Hong, S.W. Yoon, T.H. Wang, J.S. Oh, S.C. Lee, et al., J. Polym. Eng. Sci. 52, 2435–2442 (2012) H.E. Ozaytekin, G. Turedi, Ahmetli, J. Polym. Compos. 37, 3423–3432 (2016) A. Permal, M. Devarajan, H.H. Hung, T. Zahner, D. Lacey, K. Ibrahim, J. Mater. Sci. Mater. Electron. 28, 1–9 (2017) S. Nie, X. Zhang, J. Luo, Y. Liu, W. Yan, J. Polym. Composite. 38, 1–8 (2017) J. Fu, L. Shi, D. Zhang, Q. Zhong, Y. Chen, J. Polym. Eng. Sci. 50, 1809–1819 (2010) J. Wang, H. Li, G. Li, Z. Liu, J. Appl. Polym. Sci. (2017) https://doi.org/10.1002/app.44855 A.L. Feng, Z.R. Jia, Q. Yu, H.X. Zhang, G.L. Wu, Nano (2018). https://doi.org/10.1142/S1793292018500376 A.L. Feng, G.L. Wu, C. Pan, Y.Q. Wang, J. Nanosci. Nanotechnol. 17, 3859–3863 (2017)